In recent years, X-ray ptychography has been established as a valuable tool for high-resolution imaging. Nevertheless, the spatial resolution and sensitivity in coherent diffraction imaging are limited by the signal that is detected over noise and over background scattering. Especially, coherent imaging of weakly scattering specimens suffers from incoherent background that is generated by the interaction of the central beam with matter along its propagation path in particular close to and inside of the detector. Common countermeasures entail evacuated flight tubes or detector-side beamstops, which improve the experimental setup in terms of background reduction or better coverage of high dynamic range in the diffraction patterns. Here, we discuss an alternative approach: we combine two ptychographic scans with and without beamstop and reconstruct them simultaneously taking advantage of the complementary information contained in the two scans. We experimentally demonstrate the potential of this scheme for hard X-ray ptychography by imaging a weakly scattering object composed of catalytic nanoparticles and provide the analysis of the signal-to-background ratio in the diffraction patterns.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1016/j.ultramic.2016.11.005 | DOI Listing |
Nanomaterials (Basel)
January 2025
Institute of Scientific Instruments of the Czech Academy of Sciences, Kralovopolska 147, 61200 Brno, Czech Republic.
Phase contrast imaging is well-suited for studying weakly scattering samples. Its strength lies in its ability to measure how the phase of the electron beam is affected by the sample, even when other imaging techniques yield low contrast. In this study, we explore via simulations two phase contrast techniques: integrated center of mass (iCOM) and ptychography, specifically using the extended ptychographical iterative engine (ePIE).
View Article and Find Full Text PDFSmall
January 2025
Department of Chemistry, Yonsei University, Seoul, 03722, Republic of Korea.
This study reports the synthesis of plasmonic hot nanogap networks-in-triangular nanoframes (NITNFs), featuring narrow intraparticle nanogap networks embedded within triangular nanoframes. Starting from Au nanotriangles, Pt NITNFs are synthesized through a cascade reaction involving simultaneous Pt deposition and Au etching in a one-pot process. The Pt NITNFs are then transformed into plasmonically active Au NITNFs via Au coating.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
Weizmann Institute of Science, Rehovot 7610001, Israel.
We consider turbulence of waves interacting weakly via four-wave scattering (sea waves, plasma waves, spin waves, etc.). In the first order in the interaction, a closed kinetic equation has stationary solutions describing turbulent cascades.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
January 2025
William H. Miller III Department of Physics and Astronomy, The Johns Hopkins University, Baltimore, MD 21218.
Introducing an experimental technique of time-resolved inelastic neutron scattering (TRINS), we explore the time-dependent effects of resonant pulsed microwaves on the molecular magnet CrFPiv. The octagonal rings of magnetic Cr atoms with antiferromagnetic interactions form a singlet ground state with a weakly split triplet of excitations at 0.8 meV.
View Article and Find Full Text PDFChemosphere
January 2025
Institut de Chimie Séparative de Marcoule, CEA, UMR 5257 CEA-CNRS-UM-ENSCM, 30207, Bagnols-sur-Cèze, France. Electronic address:
The formation of U(VI) intrinsic colloids has a non-negligible impact on the dissemination of actinides in the environment. It is therefore essential to better identify their nature, formation conditions, and stability domains. These specific points are especially important since the behavior of these elements in environment is generally estimated by geochemical transport modeling.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!