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Revealing and Characterizing Dark Excitons through Coherent Multidimensional Spectroscopy. | LitMetric

Revealing and Characterizing Dark Excitons through Coherent Multidimensional Spectroscopy.

Phys Rev Lett

Centre for Quantum and Optical Science, Swinburne University of Technology, Hawthorn, Victoria 3122, Australia.

Published: August 2016

AI Article Synopsis

Article Abstract

Dark excitons are of fundamental importance in a broad range of contexts but are difficult to study using conventional optical spectroscopy due to their weak interaction with light. We show how coherent multidimensional spectroscopy can reveal and characterize dark states. Using this approach, we identify parity-forbidden and spatially indirect excitons in InGaAs/GaAs quantum wells and determine details regarding lifetimes, homogeneous and inhomogeneous linewidths, broadening mechanisms, and coupling strengths. The observations of coherent coupling between these states and bright excitons hint at a role for a multistep process by which excitons in the barrier can relax into the quantum wells.

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Source
http://dx.doi.org/10.1103/PhysRevLett.117.097401DOI Listing

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