In recent years, multifunctional materials contained simultaneous ferroelectric and ferromagnetic ordering have been realized. Here, a real time room temperature adaptive materials system, which demonstrates an RF magnetodielectric (MD) response, i.e., CexY3-xFe5O12 (x = 0, 0.05, 0.1, 0.15, 0.2), is reported. The magnetic and dielectric properties of Ce-doped YIG microwave ferrites processed by a traditional ceramic route have been measured over a frequency range of 4-8 GHz (C-band). The substitution of Ce not only enhances the microwave electromagnetic properties of the YIG, but also modulates the magnetodielectric response. The maximum magnetodielectric response in Ce-doped YIG sample ranges in magnitude from approximately +5% to -5% under an applied field of 1.78 kOe. This effect was attributed to electron fluctuations on the Fe cation sites. Furthermore, the magnitude of the MD response was shown to be enhanced by the cerium content. It is believed that research of the magnetodielectric effect in YIG ferrites is of great importance to the development of next generation multifunctional adaptive microwave materials, devices and integrated circuits.
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http://dx.doi.org/10.1038/srep28206 | DOI Listing |
ACS Appl Mater Interfaces
January 2025
Frontier Research Institute for Interdisciplinary Sciences, Tohoku University, Sendai 980-8578, Japan.
Spin-dependent charge tunneling transport of magnetic nanocomposites under alternating current or direct current has revolutionized the understanding of the quantum-mechanical phenomenon in complex granular solids. The tunnel magnetodielectric (TMD) and tunnel magnetoresistance (TMR) effects are two critical functionalities in this context, where dielectric permittivity and electrical resistance, respectively, change in response to an applied magnetic field due to charge tunneling. However, the structural correlation between TMD and TMR, as well as the mechanisms, remains poorly understood, largely due to the challenges in directly characterizing nanoscale intergranular interactions.
View Article and Find Full Text PDFJ Phys Condens Matter
August 2023
Key Laboratory of Polar Materials and Devices, Ministry of Education, Department of Electronics, East China Normal University, Shanghai 200241, People's Republic of China.
In this review, an overview of acoustic- and radio-frequency frequency dielectric properties of multiferroic oxides, the significant dynamic response of electrical polarization to small external ac electrical fields, are present based on the reports in literatures and our recent experimental progresses. The review is begun with some basic terms, concepts and mechanisms associated with dielectric response and dielectric anomalies, namely dielectric peak and plateau upon varying temperatures and dielectric relaxations upon varying frequencies. Subsequently, a variety of quantitative analyses and descriptions of various dielectric effects, including dielectric relaxation, relaxational and transport dynamics, ac conductivity, equivalent circuit models and impedance spectroscopy, are summarized in details.
View Article and Find Full Text PDFACS Omega
July 2023
Department of Physics, Guru Nanak Dev University, Amritsar 143005, Punjab, India.
This research study examines the high-temperature dielectric relaxation and electric conduction mechanisms in ()LaCoO-(1 - )NaBiTiO samples, where is 0.05, 0.10, and 0.
View Article and Find Full Text PDFMaterials (Basel)
January 2023
State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China.
The appearance of antiferroelectrics (AFE) in the ferrimagnetism (FM) system would give birth to a new type of multiferroic candidate, which is significant to the development of novel devices for energy storage. Here we demonstrate the realization of full antiferroelectrics in a magnetic LaSrFeO system (AFE+FM), which also presents a strong magnetodielectric response (MD) and magnetoresistance (MR) effect. The antiferroelectric phase was achieved at room temperature by replacing 0.
View Article and Find Full Text PDFNanomaterials (Basel)
August 2022
Hunan Institute of Engineering, School of Electrical and Information Engineering, Xiangtan 411104, China.
Single-phase multiferroics that allow the coexistence of ferroelectric and magnetic ordering above room temperature are highly desirable, and offer a fundamental platform for novel functionality. In this work, a double perovskite multiferroic PrFeAlO ceramic is prepared using a sol-gel process followed by a quenching treatment. The well-crystallized and purified PrFeAlO in trigonal structure with space group R3c is confirmed.
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