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| http://dx.doi.org/10.1093/swr/svw007 | DOI Listing |
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Biphasic system not only presents a promising opportunity for complex catalytic processes, but also is a grand challenge in efficient tandem reactions. As an emerging solar-to-chemical conversion, the visible-light-driven and water-donating hydrogenation combines the sustainability of photocatalysis and economic-value of hydrogenation. However, the key and challenging point is to couple water-soluble photocatalytic hydrogen evolution reaction (HER) with oil-soluble hydrogenation.
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Consecutive C-C Coupling of CH and CO Mediated by Heteronuclear Metal Cations CuTa.
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Henan Key Laboratory of Crystalline Molecular Functional Materials, College of Chemistry, Zhengzhou University, Zhengzhou 450001, China.
The conversion of methane and carbon dioxide to form C products is of great interest but presents a long-standing grand challenge due to the significant obstacle of activating the inert C-H and C═O bonds as well as forming the C-C bonds. Herein, the consecutive C-C coupling of CH and CO was realized by using heteronuclear metal cations CuTa, and the desorption of HC═C═O molecules was evidenced by state-of-the-art mass spectrometry. The CuTa reaction system is significantly different from the homonuclear metal systems of Cu and Ta.
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