Direct integration of a vertical organic field-effect transistor (VOFET) and an optoelectronic device offers a single stacked, low power optoelectronic VOFET with high aperture ratios. However, a functional optoelectronic VOFET could not be realized because of the difficulty in fabricating transparent source and gate electrodes. Here, we report a VOFET with an on/off ratio up to 10(5) as well as output current saturation by fabricating a transparent gate capacitor consisting of a perforated indium tin oxide (ITO) source electrode, HfO2 gate dielectric, and ITO gate electrode. Effects of the pore size and the pore depth within the porous ITO electrodes on the on/off characteristic of a VOFET are systematically explained in this work. By combining a phosphorescent organic light-emitting diode with an optimized VOFET structure, a vertical organic light-emitting transistor with a luminance on/off ratio of 10(4) can be fabricated.
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Anal Chim Acta
February 2025
Instituto de Química, Universidade Federal de Goiás, 74690-900, Goiânia, GO, Brazil; Instituto Nacional de Ciência e Tecnologia de Bioanalítica, Campinas, 13084-971, SP, Brazil. Electronic address:
Background: Distinct classes of environmental contaminants - such as microplastics, volatile organic compounds, inorganic gases, hormones, pesticides/herbicides, and heavy metals - have been continuously released into the environment from different sources. Anthropogenic activities with unprecedented consequences have impacted soil, surface waters, and the atmosphere. In this scenario, developing sensing materials and analytical platforms for monitoring water and air quality is essential to supporting worldwide environmental control agencies.
View Article and Find Full Text PDFNat Commun
January 2025
School of Physics, Key Laboratory of Quantum Materials and Devices of Ministry of Education, and Key Laboratory of MEMS of Ministry of Education, Southeast University, Nanjing, China.
The realization of room-temperature-operated, high-performance, miniaturized, low-power-consumption and Complementary Metal-Oxide-Semiconductor (CMOS)-compatible mid-infrared photodetectors is highly desirable for next-generation optoelectronic applications, but has thus far remained an outstanding challenge using conventional materials. Two-dimensional (2D) heterostructures provide an alternative path toward this goal, yet despite continued efforts, their performance has not matched that of low-temperature HgCdTe photodetectors. Here, we push the detectivity and response speed of a 2D heterostructure-based mid-infrared photodetector to be comparable to, and even superior to, commercial cooled HgCdTe photodetectors by utilizing a vertical transport channel (graphene/black phosphorus/molybdenum disulfide/graphene).
View Article and Find Full Text PDFNat Commun
January 2025
Department of Electrical Engineering, University of California, Irvine, CA, USA.
Complementary transistors are critical for circuits with compatible input/output signal dynamic range and polarity. Organic electronics offer biocompatibility and conformability; however, generation of complementary organic transistors requires introduction of separate materials with inadequate stability and potential for tissue toxicity, limiting their use in biomedical applications. Here, we discovered that introduction of source/drain contact asymmetry enables spatial control of de/doping and creation of single-material complementary organic transistors from a variety of conducting polymers of both carrier types.
View Article and Find Full Text PDFJ Hazard Mater
January 2025
State Key Laboratory of Water Environment Simulation, School of Environment, Beijing Normal University, Beijing 100875, China. Electronic address:
Estuarine intertidal habitats provide a dynamic and distinctive environment for the transport of microplastics, yet their migration and accumulation in these areas remain poorly understood. Herein, the spatial distribution patterns of microplastics in the estuarine sedimentary environment of the Yellow River Delta were investigated across elevation and depth gradients. Compared to the subtidal and supratidal zones, the estuarine intertidal zone exhibited the highest microplastic abundance in sediment (1027 ± 29 items/kg).
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
School of Automation Engineering, University of Electronic Science and Technology of China, Chengdu 610054, China.
Vertical organic electrochemical transistors (vOECTs) have received widespread attention in bioelectronics, wearable, and neuromorphic electronics due to their high transconductance (), low driving voltage, and biocompatibility. As key parameters of vOECTs, and switching speed (or transient time, τ) are vital for achieving satisfying performance in various practical applications. Here we employ vOECTs with varying top electrode widths for effective and switching speed modulation.
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