The non-equilibrium control of emergent phenomena in solids is an important research frontier, encompassing effects such as the optical enhancement of superconductivity. Nonlinear excitation of certain phonons in bilayer copper oxides was recently shown to induce superconducting-like optical properties at temperatures far greater than the superconducting transition temperature, Tc (refs 4-6). This effect was accompanied by the disruption of competing charge-density-wave correlations, which explained some but not all of the experimental results. Here we report a similar phenomenon in a very different compound, K3C60. By exciting metallic K3C60 with mid-infrared optical pulses, we induce a large increase in carrier mobility, accompanied by the opening of a gap in the optical conductivity. These same signatures are observed at equilibrium when cooling metallic K3C60 below Tc (20 kelvin). Although optical techniques alone cannot unequivocally identify non-equilibrium high-temperature superconductivity, we propose this as a possible explanation of our results.
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http://dx.doi.org/10.1038/nature16522 | DOI Listing |
Sci Bull (Beijing)
May 2024
State Key Laboratory of Low-Dimensional Quantum Physics, Department of Physics, Tsinghua University, Beijing 100084, China; Frontier Science Center for Quantum Information, Beijing 100084, China. Electronic address:
Magnetic impurities in superconductors are of increasing interest due to emergent Yu-Shiba-Rusinov (YSR) states and Majorana zero modes for fault-tolerant quantum computation. However, a direct relationship between the YSR multiple states and magnetic anisotropy splitting of quantum impurity spins remains poorly characterized. By using scanning tunneling microscopy, we systematically resolve individual transition-metal (Fe, Cr, and Ni) impurities induced YSR multiplets as well as their Zeeman effects in the KC superconductor.
View Article and Find Full Text PDFNano Lett
January 2020
Department of Chemistry , Pohang University of Science and Technology (POSTECH), Pohang 37673 , Republic of Korea.
Alkali metal doping is an essential process for developing organic superconductors. The conventional vapor-phase alkali metal doping, however, frequently suffers from low efficiency and poor reproducibility mainly due to the inhomogeneous reaction between alkali metal vapor and target organic molecule powder. To overcome this issue, here we developed a facile and highly reproducible solution-phase alkali metal doping (SPD) and successfully applied it to prepare potassium-doped fullerene (KC) superconductors.
View Article and Find Full Text PDFNat Phys
August 2018
Max Planck Institute for the Structure and Dynamics of Matter, Hamburg, Germany.
Nature
February 2016
Max Planck Institute for the Structure and Dynamics of Matter, Luruper Chaussee 149, 22761 Hamburg, Germany.
Molecules
April 2012
National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan.
We synthesized superconducting fullerene nanowhiskers (C(60)NWs) by potassium (K) intercalation. They showed large superconducting volume fractions, as high as 80%. The superconducting transition temperature at 17 K was independent of the K content (x) in the range between 1.
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