We investigate the thermal radiative emission of few-layer structures deposited on a metallic substrate and its dependence on temperature with the Fluctuational Electrodynamics approach. We highlight the impact of the variations of the optical properties of metallic layers on their temperature-dependent emissivity. Fabry-Pérot spectral selection involving at most two transparent layers and one thin reflective layer leads to well-defined peaks and to the amplification of the substrate emission. For a single Fabry-Pérot layer on a reflective substrate, an optimal thickness that maximizes the emissivity of the structure can be determined at each temperature. A thin lossy layer deposited on the previous structure can enhance interference phenomena, and the analysis of the participation of each layer to the emission shows that the thin layer is the main source of emission. Eventually, we investigate a system with two Fabry-Pérot layers and a metallic thin layer, and we show that an optimal architecture can be found. The total hemispherical emissivity can be increased by one order of magnitude compared to the substrate emissivity.
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http://dx.doi.org/10.1364/OE.24.00A374 | DOI Listing |
Nat Commun
December 2024
Department of Chemical Engineering, The University of Melbourne, Parkville, Victoria, Australia.
Colloidal properties of nanoparticles are intricately linked to their morphology. Traditionally, achieving high-concentration dispersions of two-dimensional (2D) nanosheets has proven challenging as they tend to agglomerate or re-stack under increased surface contact and Van der Waals attraction. Here, we unveil an excluded volume effect enabled by 2D morphology, which can be coupled with electrostatic repulsion to synthesize high-concentration aqueous graphene dispersions.
View Article and Find Full Text PDFJ Am Chem Soc
December 2024
Center for Nanochemistry, Beijing Science and Engineering Center for Nanocarbons, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, China.
The nonlinear optical response in graphene is finding increasing applications in nanophotonic devices. The activation and enhancement of second harmonic generation (SHG) in graphene, which is generally forbidden in monolayer and AB-stacked bilayer graphene due to their centrosymmetry, is of urgent need for nanophotonic applications. Here, we present a comprehensive study of SHG performance of twisted multilayer graphene structures based on stacking engineering.
View Article and Find Full Text PDFNanomaterials (Basel)
December 2024
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
Besides the intensity and wavelength, the ability to analyze the optical polarization of detected light can provide a new degree of freedom for numerous applications, such as object recognition, biomedical applications, environmental monitoring, and remote sensing imaging. However, conventional filter-integrated polarimetric sensing systems require complex optical components and a complicated fabrication process, severely limiting their on-chip miniaturization and functionalities. Herein, the reconfigurable polarimetric photodetection with photovoltaic mode is developed based on a few-layer MoS/PdSe heterostructure channel and a charge-trap structure composed of AlO/HfO/AlO (AHA)-stacked dielectrics.
View Article and Find Full Text PDFNanoscale
December 2024
Boston University, Department of Mechanical Engineering, Boston, MA 02215, USA.
We measure the out-of-plane shear modulus of few-layer graphene (FLG) by a blister test. During the test, we employed a monolayer molybdenum disulfide (MoS) membrane stacked onto FLG wells to facilitate the separation of FLG from the silicon oxide (SiO) substrate. Using the deflection profile of the blister, we determine an average shear modulus of 0.
View Article and Find Full Text PDFNanophotonics
August 2024
School of Physics, State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China.
Platinum diselenide (PtSe), classified as a noble metal dichalcogenide, has garnered substantial interest owing to its layer-dependent band structure, remarkable air-stability, and high charge-carrier mobilities. These properties make it highly promising for a wide array of applications in next-generation electronic and optoelectronic devices, as well as sensors. Additionally, two-dimensional (2D) PtSe demonstrates significant potential as a saturable absorber due to its exceptional nonlinear optical response across an ultrabroad spectra range, presenting exciting opportunities in ultrafast and nonlinear photonics.
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