The absorption of ultraintense, femtosecond laser pulses by a solid unleashes relativistic electrons, thereby creating a regime of relativistic optics. This has enabled exciting applications of relativistic particle beams and coherent X-ray radiation, and fundamental leaps in high energy density science and laboratory astrophysics. Obviously, central to these possibilities lies the basic problem of understanding and if possible, manipulating laser absorption. Surprisingly, the absorption of intense light largely remains an open question, despite the extensive variations in target and laser pulse structures. Moreover, there are only few experimental measurements of laser absorption carried out under very limited parameter ranges. Here we present an extensive investigation of absorption of intense 30 femtosecond laser pulses by solid metal targets. The study, performed under varying laser intensity and contrast ratio over four orders of magnitude, reveals a significant and non-intuitive dependence on these parameters. For contrast ratio of 10(-9) and intensity of 2 × 10(19)W cm(-2), three observations are revealed: preferential acceleration of electrons along the laser axis, a ponderomotive scaling of electron temperature, and red shifting of emitted second-harmonic. These point towards the role of J × B absorption mechanism at relativistic intensity. The experimental results are supported by particle-in-cell simulations.
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http://dx.doi.org/10.1038/srep17870 | DOI Listing |
Sci Rep
January 2025
Department of Chemical Engineering, Faculty of Engineering, Mahidol University, Phuttamonthon 4 Road, Nakhon Pathom, 73170, Thailand.
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View Article and Find Full Text PDFLuminescence
January 2025
College of Science, Sichuan Agricultural University, Ya'an, Sichuan, China.
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View Article and Find Full Text PDFInt J Biol Macromol
January 2025
Key Laboratory of Bio-based Material Science & Technology (Ministry of Education), Northeast Forestry University, Harbin 150040, China; College of Material Science and Engineering, Northeast Forestry University, Harbin 150040, China.
Carboxymethyl chitosan (CMCh) is a natural polysaccharide derivative with biodegradability, rich in active amino and carboxyl groups. It can act as a ligand to coordinate with rare earth ions, transferring absorbed energy to the central ion to sensitize its luminescence. In this paper, CMCh-Tb was prepared as a solid fluorescent probe by mixing CMCh solution with Tb.
View Article and Find Full Text PDFJ Phys Chem A
January 2025
Department of Chemistry, Louisiana State University, Baton Rouge, Louisiana 70803, United States.
When dielectrics are hit with intense infrared (IR) laser pulses, transient metalization can occur. The initial attosecond dynamics behind this metallization are not entirely understood. Therefore, simulations are needed to understand this process and to help interpret experimental observations of it, such as with attosecond transient absorption (ATA).
View Article and Find Full Text PDFHeliyon
January 2025
Department of Pharmaceutical Chemistry, College of Pharmacy King Saud University, Riyadh Saudi Arabia.
In this study, an optical sensor, JA/(2,6-di((E)-benzylidene)cyclohexan-1-one), was synthesized and characterized using H NMR and FT-IR spectroscopy. The sensor exhibited high efficiency and selectivity in detecting Pb ions, even in the presence of potential interfering ions such as Mn, Cu, Co, Cr, Ni, Ce, Hg, and Cd in aqueous solutions. The interaction of JA with Pb resulted in a significant enhancement of fluorescence intensity, suggesting the formation of a stable complex.
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