By means of neutron scattering and magnetization measurements down to 90 mK, we determine the magnetic ground state of the spin-ice candidate Nd(2)Zr(2)O(7). We show that, despite ferromagnetic interactions, Nd(2)Zr(2)O(7) undergoes a transition around 285 mK towards an all-in-all-out antiferromagnetic state, with a strongly reduced ordered magnetic moment. We establish the (H,T) phase diagram in the three directions of the applied field and reveal a metamagnetic transition around 0.1 T, associated with an unexpected shape of the magnetization curves. We propose that this behavior results from the peculiar nature of the Nd^{3+} doublet, a dipolar-octupolar doublet, different from the standard Kramers doublet studied to date, thus revealing the importance of multipolar correlations in the properties of pyrochlore oxides.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1103/PhysRevLett.115.197202 | DOI Listing |
Nat Commun
November 2024
Department of Physics and Astronomy, Rutgers University, Piscataway, NJ, USA.
Nat Commun
July 2018
Division of Physics, Mathematics, and Astronomy, California Institute of Technology, Pasadena, CA, 91125, USA.
Dimensionality and symmetry play deterministic roles in the laws of Nature. They are important tools to characterize and understand quantum phase transitions, especially in the limit of strong correlations between spin, orbit, charge, and structural degrees of freedom. Here, using newly-developed, high-pressure resonant X-ray magnetic and charge diffraction techniques, we have discovered a quantum critical point in CdOsO as the all-in-all-out antiferromagnetic order is continuously suppressed to zero temperature and, concomitantly, the cubic lattice structure continuously changes from space group Fd-3m to F-43m.
View Article and Find Full Text PDFNat Commun
July 2016
Department of Physics and Astronomy, University of Waterloo, Waterloo, Ontario, Canada N2L 3G1.
We present a new classical spin liquid on the pyrochlore lattice by extending spin ice with further neighbour interactions. We find that this disorder-free spin model exhibits a form of dynamical heterogeneity with extremely slow relaxation for some spins, while others fluctuate quickly down to zero temperature. We thus call this state spin slush, in analogy to the heterogeneous mixture of solid and liquid water.
View Article and Find Full Text PDFPhys Rev Lett
November 2015
Department of Physics, University of Warwick, Coventry, CV4 7AL, United Kingdom.
By means of neutron scattering and magnetization measurements down to 90 mK, we determine the magnetic ground state of the spin-ice candidate Nd(2)Zr(2)O(7). We show that, despite ferromagnetic interactions, Nd(2)Zr(2)O(7) undergoes a transition around 285 mK towards an all-in-all-out antiferromagnetic state, with a strongly reduced ordered magnetic moment. We establish the (H,T) phase diagram in the three directions of the applied field and reveal a metamagnetic transition around 0.
View Article and Find Full Text PDFPhys Rev Lett
July 2012
Physik-Department E21, Technische Universität München, D-85748 Garching, Germany.
We have explored the spin liquid state in Tb(2)Ti(2)O(7) with vibrating-coil magnetometry down to ~0.04 K under magnetic fields up to 5 T. We observe magnetic history dependence below T*~0.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!