Alpha spectrometry applications with mass separated samples.

Appl Radiat Isot

Pacific Northwest National Laboratory Richland, WA 99354, United States.

Published: January 2016

(241)Am has been deposited using a novel technique that employs a commercial inductively coupled plasma mass spectrometer. This work presents results of high-resolution alpha spectrometry on the (241)Am samples using a small area passivated implanted planar silicon detector. We have also investigated the mass-based separation capability by developing a (238)Pu sample, present as a minor constituent in a (244)Pu standard, and performed subsequent radiometric counting. With this new sample development method, the (241)Am samples achieved the intrinsic energy resolution of the detector used for these measurements. There was no detectable trace of any other isotopes contained in the (238)Pu implant demonstrating the mass-based separation (or enhancement) attainable with this technique.

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http://dx.doi.org/10.1016/j.apradiso.2015.09.013DOI Listing

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