We present a formulation of the model of laser-plasma interaction (LPI) at hydrodynamical scales that couples the plasma dynamics with linear and nonlinear LPI processes, including the creation and propagation of high-energy electrons excited by parametric instabilities and collective effects. This formulation accounts for laser beam refraction and diffraction, energy absorption due to collisional and resonant processes, and hot electron generation due to the stimulated Raman scattering, two-plasmon decay, and resonant absorption processes. Hot electron (HE) transport and absorption are described within the multigroup angular scattering approximation, adapted for transversally Gaussian electron beams. This multiscale inline LPI-HE model is used to interpret several shock ignition experiments, highlighting the importance of target preheating by HEs and the shortcomings of standard geometrical optics when modeling the propagation and absorption of intense laser pulses. It is found that HEs from parametric instabilities significantly increase the shock pressure and velocity in the target, while decreasing its strength and the overall ablation pressure.
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http://dx.doi.org/10.1103/PhysRevE.92.041101 | DOI Listing |
Anal Chim Acta
March 2025
Zhejiang Key Laboratory of Advanced Optical Functional Materials and Devices, Ningbo University, Ningbo, 315211, China; Engineering Research Center for Advanced Infrared Photoelectric Materials and Devices of Zhejiang Province, Ningbo University, Ningbo, 315211, China. Electronic address:
Background: Permethrin is a pesticide used to kill insects, and once used in excess, it poses a great threat to the environment and human health, therefore, it is necessary to realize the rapid and accurate detection of permethrin. Fiber optic surface enhanced Raman scattering (SERS) probes have the advantages of small volume and can be used for remote monitoring, which have great potential for application in achieving in-situ detection of pesticide residues.
Results: Fiber taper waist (FTW) SERS probes modified by silver nanocubes-graphene oxide (Ag NCs-GO) composite structures were prepared for in situ detection of permethrin in lake water.
Int J Biol Macromol
January 2025
Key Laboratory of State Administration of Traditional Chinese Medicine, Dongguan HEC Cordyceps R&D Co., Ltd., Dongguan, Guangdong 523850, China; College of Medical Imaging Laboratory and Rehabilitation, Xiangnan University, Chenzhou, Hunan 423000, China. Electronic address:
Cultivated Chinese cordyceps, an optimal substitute for the endangered wild resource, has recently been produced on a large scale. This work sought to explore the structural features and immunomodulatory activity of a novel low-molecular-weight polysaccharide (CSP1a, 15.7 kDa) isolated from cultivated Chinese cordyceps.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
February 2025
Department of Biosphere Sciences and Engineering, Carnegie Institution for Science, Stanford, CA 94305.
Microbial mats are stratified communities often dominated by unicellular and filamentous phototrophs within an exopolymer matrix. It is challenging to quantify the dynamic responses of community members in situ as they experience steep gradients and rapid fluctuations of light. To address this, we developed a binary consortium using two representative isolates from hot spring mats: the unicellular oxygenic phototrophic cyanobacterium OS-B' (Syn OS-B') and the filamentous anoxygenic phototroph MS-CIW-1 (Chfl MS-1).
View Article and Find Full Text PDFJ Chem Phys
January 2025
Department of Chemistry, Princeton University, Princeton, New Jersey 08544, USA.
Time-resolved spectroscopy is an important tool for probing photochemically induced nonequilibrium dynamics and energy transfer. Herein, a method is developed for the ab initio simulation of vibronic spectra and dynamical processes. This framework utilizes the recently developed nuclear-electronic orbital time-dependent configuration interaction (NEO-TDCI) approach, which treats all electrons and specified nuclei quantum mechanically on the same footing.
View Article and Find Full Text PDFNanoscale
January 2025
Department of Chemistry, Maulana Azad National Institute of Technology, Bhopal-462003, India.
Mixing different metal ions at the B site of ABX perovskites offers a promising approach for addressing challenges related to toxicity, stability and performance in optoelectronic applications. One such example is CsPbSnBr which addresses the toxicity issue posed by lead while allowing us to tune optoelectronic properties such as the band gap. In this work, nearly monodisperse CsPbSnBr quantum dots (QDs) were synthesized with variable Pb/Sn compositions, CsPbBr, CsPbSnBr and CsPbSnBr.
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