Topological insulators (TIs) are a new class of quantum materials that exhibit a current-induced spin polarization due to spin-momentum locking of massless Dirac Fermions in their surface states. This helical spin polarization in three-dimensional (3D) TIs has been observed using photoemission spectroscopy up to room temperatures. Recently, spin polarized surface currents in 3D TIs were detected electrically by potentiometric measurements using ferromagnetic detector contacts. However, these electric measurements are so far limited to cryogenic temperatures. Here we report the room temperature electrical detection of the spin polarization on the surface of Bi2Se3 by employing spin sensitive ferromagnetic tunnel contacts. The current-induced spin polarization on the Bi2Se3 surface is probed by measuring the magnetoresistance while switching the magnetization direction of the ferromagnetic detector. A spin resistance of up to 70 mΩ is measured at room temperature, which increases linearly with current bias, reverses sign with current direction, and decreases with higher TI thickness. The magnitude of the spin signal, its sign, and control experiments, using different measurement geometries and interface conditions, rule out other known physical effects. These findings provide further information about the electrical detection of current-induced spin polarizations in 3D TIs at ambient temperatures and could lead to innovative spin-based technologies.
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http://dx.doi.org/10.1021/acs.nanolett.5b03080 | DOI Listing |
J Phys Condens Matter
December 2024
Department of Physics and Astronomy, University of Nebraska-Lincoln, Jorgenesen Hall, 855 North 16th Street, Lincoln, Nebraska, 68588-0299, UNITED STATES.
Evidence of chirality was observed at the Fe metal center in Fe(III) spin crossover coordination salts [Fe(qsal)Ni(dmit)] and [Fe(qsal)(TCNQ)] from X-ray absorption spectroscopy at the Fe 2pcore threshold. Based on the circularly polarized X-ray absorption data, the X-ray natural circular dichroism seen [Fe(qsal)Ni(dmit)] and [Fe(qsal)(TCNQ)] is far stronger than seen for [Fe(qsal)Cl] suggesting this natural circular dichroism signature is a ligand effect rather than a result of just a loss of octahedral symmetry on the Fe core. The larger the chiral effects in the Fe 2p core to bound X-ray absorption, the greater the perturbation of the Fe 2pto 2pspin-orbit splitting seen in the X-ray absorption spectra.
View Article and Find Full Text PDFPolarization ellipses are well-known as the result of coherent superposition of photonic spin states. As orbital counterparts, in this Letter, we introduce centroid ellipses that are geometrically mapped from optical orbital angular momentum (OAM) superpositions on a modal Poincaré sphere (PS) by coaxial interference. Different from not easily observable polarization ellipses, these centroid ellipses can be directly observed from dynamical interferograms with broken rotational symmetry.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
Department of Physics and Astronomy, University College London, Gower Street, London WC1E 6BT, United Kingdom.
We have measured the spin polarization of a slow positron beam via state-selective depopulation of 2^{3}S_{1} positronium atoms, generated by passing the beam through a gas cell. Our method employs circularly polarized microwave radiation to drive 2^{3}S_{1}→2^{3}P_{1} transitions, for which either Δm_{J}=+1 or Δm_{J}=-1, and relies on the fact that asymmetries between the two cases yield the underlying positron beam polarization. Using this technique we show that the polarization of a positron beam derived from a solid neon moderator may be increased from 30% to 90% by increasing the moderator thickness, with an associated reduction in beam intensity of 60%.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
Center for Quantum Spintronics, Department of Physics, Norwegian University of Science and Technology, NO-7491 Trondheim, Norway.
New unconventional compensated magnets with a p-wave spin polarization protected by a composite time-reversal translation symmetry have been proposed in the wake of altermagnets. To facilitate the experimental discovery and applications of these unconventional magnets, we construct an effective analytical model. The effective model is based on a minimal tight-binding model for unconventional p-wave magnets that clarifies the relation to other magnets with p-wave spin-polarized bands.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
December 2024
South China University of Technology School of Materials Science and Engineering, State Key Laboratory of Luminescent Materials and Devices and Institute of Polymer Optoelectronic Materials and Devices, 381 Wushan Road, 510640, Guangzhou, CHINA.
The exploration of circularly polarized luminescence is important for advancing display and lighting technologies. Herein, by utilizing isomeric molecular engineering, a novel series of chiral molecules are designed to exploit both thermally activated delayed fluorescence (TADF) and room-temperature phosphorescence (RTP) mechanisms for efficient luminescence. The cooperation of a small singlet-triplet energy gap, moderate spin-orbital coupling (SOC), and large oscillator strength enables efficient TADF emission, with photoluminescence quantum yields exceeding 90%.
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