Nanoscale and Single-Dot Patterning of Colloidal Quantum Dots.

Nano Lett

Physics and Chemistry of Nanostructures, Ghent University, Krijgslaan 281-S3, 9000 Ghent, Belgium.

Published: November 2015

Using an optimized lift-off process we develop a technique for both nanoscale and single-dot patterning of colloidal quantum dot films, demonstrating feature sizes down to ~30 nm for uniform films and a yield of 40% for single-dot positioning, which is in good agreement with a newly developed theoretical model. While first of all presenting a unique tool for studying physics of single quantum dots, the process also provides a pathway toward practical quantum dot-based optoelectronic devices.

Download full-text PDF

Source
http://dx.doi.org/10.1021/acs.nanolett.5b03068DOI Listing

Publication Analysis

Top Keywords

nanoscale single-dot
8
single-dot patterning
8
patterning colloidal
8
colloidal quantum
8
quantum dots
8
quantum
4
dots optimized
4
optimized lift-off
4
lift-off process
4
process develop
4

Similar Publications

Article Synopsis
  • The study investigates how carriers behave in CdSe/ZnS quantum dots using fluorescence-lifetime-correlation-spectroscopy (FLCS) and single-dot photoluminescence (PL) blinking.
  • It distinguishes between the emission of photons from exciton and trap states by analyzing their lifetimes and establishes correlation functions that reveal similar diffusion times across both states.
  • The findings suggest that different states contribute to the blinking phenomenon, with shallow trap states dominating at lower excitation powers and trion recombination influencing behavior at higher powers, showcasing the potential for a comprehensive understanding of charge dynamics in these quantum dots.
View Article and Find Full Text PDF

Metal halide semicondictor perovskites have been under intense investigation for their promise in light absorptive applications like photovoltaics. They have more recently experienced interest for their promise in light emissive applications. A key aspect of perovskites is their glassy, ionic lattice that exhibits dynamical disorder.

View Article and Find Full Text PDF

Featured with its extraordinary super-resolution capability, the advent of stimulated emission depletion (STED) lithography has allowed for vastly reduced minimum feature size of a single pixel down to the deep sub-diffraction scale so as to produce unprecedented nanofeatures. However, the anticipated sub-diffraction pixel pitch down below 100 nm remains out of reach due to redundant polymerization of adjacent exposures at a short distance, so called memory effect. In this work, a nanoprinting-at-expansion/employments-at-recovery strategy is applied in the dual-beam STED lithography technique to surmount the memory effect and break adjacent-exposure limit imposed on minimizing the pixel pitch.

View Article and Find Full Text PDF

Giant shell CdSe/CdS quantum dots are bright and flexible emitters, with near-unity quantum yield and suppressed blinking, but their single photon purity is reduced by efficient multiexcitonic emission. We report the observation, at the single dot level, of a large blueshift of the photoluminescence biexciton spectrum (24 ± 5 nm over a sample of 32 dots) for pure-phase wurtzite quantum dots. By spectral filtering, we demonstrate a 2.

View Article and Find Full Text PDF

The trade-off between the functionalization shift of the informative parameters and sensitivity of capacitive micromachined ultrasound transducers (CMUT)-based CO sensors is addressed, and the CMUT surface modification process by thin inkjet-printed polyethyleneimine (PEI) films is optimized. It was shown that by the proper preparation of the active CMUT surface and properly diluted PEI solution, it is possible to minimize the functionalization shift of the resonance frequency and the quality of the resonance and preserve the sensitivity potential. So, after optimization, we demonstrated 23.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!