We show that graphene possesses a strong nonlinear optical response in the form of multiplasmon absorption, with exciting implications in classical and quantum nonlinear optics. Specifically, we predict that graphene nanoribbons can be used as saturable absorbers with low saturation intensity in the far-infrared and terahertz spectrum. Moreover, we predict that two-plasmon absorption and extreme localization of plasmon fields in graphene nanodisks can lead to a plasmon blockade effect, in which a single quantized plasmon strongly suppresses the possibility of exciting a second plasmon.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1103/PhysRevLett.114.236801 | DOI Listing |
Phys Rev E
November 2023
GoLP / IPFN, Instituto Superior Técnico, Universidade de Lisboa, Av. Rovisco Pais 1, 1049-001 Lisboa, Portugal.
We study the dispersion properties of electron plasma waves, or plasmons, which can be excited in quantum plasmas in the nonlinear regime. In order to describe nonlinear electron response to finite amplitude plasmons, we apply the Volkov approach to nonrelativistic electrons. For that purpose, we use the Schrödinger equation and describe the electron population of a quantum plasma as a mixture of quantum states.
View Article and Find Full Text PDFNanophotonics
September 2022
Faculty of Physics and Center for Nanointegration, Duisburg-Essen (CENIDE), University of Duisburg-Essen, 47048 Duisburg, Germany.
Spectroscopic photoemission microscopy is used to detect and quantify a ponderomotive shift in the energy of electrons that are emitted from a surface plasmon polariton focus. The focus is formed on an atomically flat Au(111) surface by an Archimedean spiral and is spatiotemporally separated from the circularly polarized light pulse used to excite the spiral. A spectroscopic analysis of electrons emitted from the focus exhibits a peaked above-threshold electron emission spectrum.
View Article and Find Full Text PDFRSC Adv
June 2022
School of Energy Science and Engineering, Central South University Changsha Hunan 410083 China
Solar selective absorbers influence the photothermal efficiency of high-temperature solar thermal applications directly and significantly. In present work, a metasurface absorber consisting of an octagonal prism array is proposed, optimized and analyzed. Firstly, the structure parameters of the absorber are optimized, finding the optimal absorber achieves near-perfect spectrally-selectivity compared with the perfect solar absorber.
View Article and Find Full Text PDFThis paper shows a strategy to realize ultra-broadband absorption of multi-spectral coverage. A vertical cascaded plasmonic absorber constructed by multilayer helical metallic nanostructure wrapped in a pyramid-shaped dielectric jacket is presented and investigated by numerical simulations. By premeditated planning of the scale proportions of the spirals and the dimension size of the pyramid-shaped dielectric, more than 90% of absorption is realized in 189-3896 nm, an ultra-wide spectral range that basically covers the bands of near-ultraviolet, visible light, and near-infrared.
View Article and Find Full Text PDFNanoscale
September 2019
CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, China. and University of Chinese Academy of Sciences, Beijing 100049, China.
One of the critical challenges for semiconductor photocatalysis is the high efficiency utilization of solar energy. For plasmonic metal-semiconductor photocatalysts, the photocatalytic activity over an extended wavelength range for a photoresponsive semiconductor could be significantly improved either via the direct electron transfer (DET) or via the plasmon-induced resonant energy transfer (PIRET). Still, the narrow spectral overlap of plasmon and the semiconductor band edge is a key factor in restricting the development of PIRET.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!