An outflow of continental haze occurs from Indo-Gangetic Basin (IGB) in the North to Bay of Bengal (BoB) in the South. An integrated campaign was organized to investigate this continental haze during December 2013-February 2014 at source and remote regions within IGB to quantify its radiative effects. Measurements were carried out at three locations in eastern India; 1) Kalas Island, Sundarban (21.68°N, 88.57°E) - an isolated island along the north-east coast of BoB, 2) Kolkata (22.57°N, 88.42°E) - an urban metropolis and 3) Siliguri (26.70°N, 88.35°E) - an urban region at the foothills of eastern Himalayas. Ground-based AOD (at 0.5 μm) is observed to be maximum (1.25±0.18) over Kolkata followed by Siliguri (0.60±0.17) and minimum over Sundarban (0.53±0.18). Black carbon concentration is found to be maximum at Kolkata (21.6±6.6 μg·m(-3)) with almost equal concentrations at Siliguri (12.6±5.2 μg·m(-3)) and Sundarban (12.3±3.0 μg·m(-3)). Combination of MODIS-AOD and back-trajectories analysis shows an outflow of winter-time continental haze originating from central IGB and venting out through Sundarban towards BoB. This continental haze with high extinction coefficient is identified up to central BoB using CALIPSO observations and is found to contribute ~75% to marine AOD over central BoB. This haze produces significantly high aerosol radiative forcing within the atmosphere over Kolkata (75.4 Wm(-2)) as well as over Siliguri and Sundarban (40 Wm(-2)) indicating large forcing over entire IGB, from foothills of the Himalayas to coastal region. This winter-time continental haze also causes about similar radiative heating (1.5 K·day(-1)) from Siliguri to Sundarban which is enhanced over Kolkata (3 K·day(-1)) due to large emission of local urban aerosols. This high aerosol heating over entire IGB and coastal region of BoB can have considerable impact on the monsoonal circulation and more importantly, such haze transported over to BoB can significantly affect the marine hydrological cycle.
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http://dx.doi.org/10.1016/j.scitotenv.2015.06.085 | DOI Listing |
Proc Natl Acad Sci U S A
July 2024
Key Laboratory of Cluster Science, Ministry of Education of China, School of Chemistry and Chemical Engineering, Beijing Institute of Technology, Beijing 100081, China.
Environ Sci Process Impacts
June 2024
State Key Laboratory of Loess and Quaternary Geology, CAS Center for Excellence in Quaternary Science and Global Change, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an 710061, China.
Vertical observations of atmospheric pollutants play crucial roles in a comprehensive understanding of the distribution characteristics and transport of atmospheric pollutants. A hexacopter uncrewed aerial vehicle equipped with miniature monitors was employed to measure the vertical distribution of atmospheric pollutants within a height of 1000 m at a rural site in Xi'an, China, in 2021. The concentrations of carbon monoxide (CO) and particulate matter (PM) showed generally decreasing trends with increasing height.
View Article and Find Full Text PDFJ Environ Manage
November 2023
State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China; Shaanxi Provincial Key Laboratory of Accelerator Mass Spectrometry Technology and Application, Xi'an AMS Center, Xi'an, 710061, China.
Radiocarbon (C), stable carbon isotope (C), and levoglucosan in PM were measured in two northern Chinese cities during haze events and nonhaze periods in January 2019, to ascertain the sources and their differences in carbonaceous aerosols between the two periods. The contribution of primary vehicle emissions (17.8 ± 3.
View Article and Find Full Text PDFSci Total Environ
February 2023
School of Earth and Environmental Sciences, Seoul National University, Seoul 08826, Republic of Korea. Electronic address:
Despite the curtailment of atmospheric condensing precursor gases during the Coronavirus disease 2019 (COVID-19) lockdown (LD) period, unexpected haze events via the formation of new particles and their subsequent growth have been identified. This study investigated the impact of emission reduction during the Chinese LD period on the new particle formation (NPF) frequency and corresponding particle number size distribution (PNSD) at three regional background atmospheric monitoring sites in the western coastal areas of the Korean Peninsula. During this duration, the number concentrations of the nucleation- (<25 nm) and accumulation-mode (>90 nm) particles significantly decreased in Baengryeong (BRY), showing decreases of 34% and 29%, respectively.
View Article and Find Full Text PDFSci Total Environ
November 2022
Chubu Institute for Advanced Studies, Chubu University, Kasugai 487-8501, Japan.
The widespread haze pollution over South Asia typically occurs in winter, affecting the abundance of organic aerosols (OA) over the Arabian Sea due to prevailing meteorology. We determined the concentrations of biomass burning (BB) derived anhydrosugars (levoglucosan: Lev, galactosan: Gal, and mannosan: Man), sugars (glucose, fructose, sucrose, and trehalose) and sugar alcohols (arabitol, mannitol, erythritol, and inositol) over the Arabian Sea during a winter cruise (6-24 December 2018). Molecular distributions revealed predominance of levoglucosan or sucrose.
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