Geological activity is thought to be important for the origin of life and for maintaining planetary habitability. We show that transient sulfate aerosols could be a signature of exoplanet volcanism and therefore of a geologically active world. A detection of transient aerosols, if linked to volcanism, could thus aid in habitability evaluations of the exoplanet. On Earth, subduction-induced explosive eruptions inject SO2 directly into the stratosphere, leading to the formation of sulfate aerosols with lifetimes of months to years. We demonstrate that the rapid increase and gradual decrease in sulfate aerosol loading associated with these eruptions may be detectable in transit transmission spectra with future large-aperture telescopes, such as the James Webb Space Telescope (JWST) and European Extremely Large Telescope (E-ELT), for a planetary system at a distance of 10 pc, assuming an Earth-like atmosphere, bulk composition, and size. Specifically, we find that a signal-to-noise ratio of 12.1 and 7.1 could be achieved with E-ELT (assuming photon-limited noise) for an Earth analogue orbiting a Sun-like star and M5V star, respectively, even without multiple transits binned together. We propose that the detection of this transient signal would strongly suggest an exoplanet volcanic eruption, if potential false positives such as dust storms or bolide impacts can be ruled out. Furthermore, because scenarios exist in which O2 can form abiotically in the absence of volcanic activity, a detection of transient aerosols that can be linked to volcanism, along with a detection of O2, would be a more robust biosignature than O2 alone.
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http://dx.doi.org/10.1089/ast.2014.1204 | DOI Listing |
J Phys Chem A
January 2025
School of Chemistry, University of Bristol, Bristol BS8 1TS, U.K.
In both nature and industry, aerosol droplets contain complex mixtures of solutes, which in many cases include multiple inorganic components. Understanding the drying kinetics of these droplets and the impact on resultant particle morphology is essential for a variety of applications including improving inhalable drugs, mitigating disease transmission, and developing more accurate climate models. However, the previous literature has only focused on the relationship between drying kinetics and particle morphology for aerosol droplets containing a single nonvolatile component.
View Article and Find Full Text PDFEnviron Pollut
December 2024
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China; College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing, 100049, China.
A multiple-site filter-sampling observation study was conducted in a coastal industrial city (Rizhao, 35°10'59″N, 119°23'57″E) to understand the main components, formation mechanisms, and potential sources of particulate matter. The average (±σ) mass concentration of PM across all the sites was 42 (±27) μg/m, with high variability (6-202 μg/m). Water-soluble inorganic ions (WSIIs) were the major contributors (54%-60%) to PM with mean values for sulfate (13 μg/m), nitrate (6 μg/m), and ammonium (7 μg/m) (SNA).
View Article and Find Full Text PDFSurg Infect (Larchmt)
December 2024
Department of Hepatobiliary and Pancreatic Surgery, Shulan (Hangzhou) Hospital, Hangzhou, P.R. China.
This study intended to evaluate the clinical efficacy and safety of colistin sulfate aerosol inhalation in combination with ceftazidime-avibactam for the treatment of pulmonary carbapenem-resistant (CRKP) infection during the peri-operative period of liver transplantation. A retrospective analysis was designed to investigate 52 patients who developed pulmonary CRKP infection after liver transplantation between December 1, 2019, and November 30, 2022. On the basis of whether they received colistin sulfate aerosol inhalation, the patients were divided into the treatment group ( = 29) and the control group ( = 23).
View Article and Find Full Text PDFJ Environ Manage
January 2025
Department of Civil Engineering, Indian Institute of Technology Indore, Simrol, Indore, 453552, Madhya Pradesh, India. Electronic address:
Extreme air pollution poses global health and environmental threats, necessitating robust policy interventions. This study first analyses the surface mass concentration of major aerosols (such as black carbon, organic carbon, dust, sea salts, and sulphates) to estimate global PM concentrations from 1980 to 2023. The developed model-estimated PM database was validated against data from 526 cities worldwide, showing strong accuracy, with RMSE, r, and R values of 7.
View Article and Find Full Text PDFACS Earth Space Chem
December 2024
Université Paris-Est Créteil and Université Paris Cité, CNRS, LISA, Créteil F-94010, France.
Hydroxyacetone (HA) is an atmospheric oxidation product of isoprene and other organic precursors that can form brown carbon (BrC). Measured bulk aqueous-phase reaction rates of HA with ammonium sulfate, methylamine, and glycine suggest that these reactions cannot compete with aqueous-phase hydroxyl radical oxidation. In cloud chamber photooxidation experiments with either gaseous or particulate HA in the presence of the same N-containing species, BrC formation was minor, with similar mass absorption coefficients at 365 nm (<0.
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