Simultaneous removal of PCDD/Fs and NOx from the flue gas of a municipal solid waste incinerator with a pilot plant.

Chemosphere

Beijing Engineering Research Center of Process Pollution Control, National Engineering Laboratory for Hydrometallurgical Cleaner Production Technology, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China. Electronic address:

Published: August 2015

The pilot-scale plant on the simultaneous removal of PCDD/Fs and NOx from the flue gas of a municipal solid waste incinerator is presented. In order to research the influence of temperature on the catalytic decomposition of PCDD/Fs and the selective catalytic reduction of NOx, the experiments were performed at 220 °C, 260 °C, and 300 °C, and the congener profiles of PCDD/Fs for the samples collected at the inlet and outlet were illustrated. Noteworthy, the detailed congener distributions of PCDD/Fs in the gas-phase and particle-phase of the inlet and 300-outlet (decomposition temperature = 300 °C) samples are presented, and the removal efficiencies η(g-I-TEQ) and η(p-I-TEQ) reached to 94.94% and 99.67%, respectively. The effect of the SCR process on the removal of PCDD/Fs was also studied at a relatively low temperature of 220 °C. Additionally, the NOx emissions and the SCR efficiencies were investigated.

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http://dx.doi.org/10.1016/j.chemosphere.2015.04.009DOI Listing

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