Strong localization effect and carrier relaxation dynamics in self-assembled InGaN quantum dots emitting in the green.

Nanoscale Res Lett

Department of Electronic Engineering, Optoelectronics Engineering Research Center, Xiamen University, 422 South Siming Road, Xiamen, 361005 P. R. China.

Published: April 2015

AI Article Synopsis

  • The study shows that InGaN quantum dots exhibit a strong localization effect, impacting their emission properties when temperature and excitation power vary.
  • At higher temperatures (up to 160 K) and high excitation intensities, there’s a notable increase in emission intensity and internal quantum efficiency, while low excitation intensity does not show this effect.
  • The research introduces a strong localization model to explain carrier movement and recombination processes, as well as employing a biexponential model for analyzing time-resolved photoluminescence data, providing insights into carrier relaxation dynamics.

Article Abstract

Strong localization effect in self-assembled InGaN quantum dots (QDs) grown by metalorganic chemical vapor deposition has been evidenced by temperature-dependent photoluminescence (PL) at different excitation power. The integrated emission intensity increases gradually in the range from 30 to 160 K and then decreases with a further increase in temperature at high excitation intensity, while this phenomenon disappeared at low excitation intensity. Under high excitation, about 40% emission enhancement at 160 K compared to that at low temperature, as well as a higher internal quantum efficiency (IQE) of 41.1%, was observed. A strong localization model is proposed to describe the possible processes of carrier transport, relaxation, and recombination. Using this model, the evolution of excitation-power-dependent emission intensity, shift of peak energy, and linewidth variation with elevating temperature is well explained. Finally, two-component decays of time-resolved PL (TRPL) with various excitation intensities are observed and analyzed with the biexponential model, which enables us to further understand the carrier relaxation dynamics in the InGaN QDs.

Download full-text PDF

Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC4384949PMC
http://dx.doi.org/10.1186/s11671-015-0772-zDOI Listing

Publication Analysis

Top Keywords

strong localization
12
carrier relaxation
8
relaxation dynamics
8
self-assembled ingan
8
ingan quantum
8
quantum dots
8
emission intensity
8
high excitation
8
excitation intensity
8
temperature well
8

Similar Publications

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!