Efficient collection of the broadband fluorescence from the diamond nitrogen vacancy (NV) center is essential for a range of applications in sensing, on-demand single photon generation, and quantum information processing. Here, we introduce a circular "bullseye" diamond grating which enables a collected photon rate of (2.7 ± 0.09) × 10(6) counts per second from a single NV with a spin coherence time of 1.7 ± 0.1 ms. Back-focal-plane studies indicate efficient redistribution of the NV photoluminescence into low-NA modes by the bullseye grating.
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Environ Sci Pollut Res Int
January 2025
Department of Chemistry, Laboratory of Catalysis, Environment and Materials, State University of Rio Grande Do Norte, 59610-210, Mossoró, Rio Grande Do Norte, Brazil.
In this study, a novel synthesis approach was employed to create the KIT-6/TiO photocatalyst with different ratios of Si/Ti. The results of the X-ray diffraction revealed that incorporating TiO with the anatase phase maintained the mesoporous structure of KIT-6 (Korean Institute of Technology 6). The scanning electron microscope and transmission electron microscope images exhibited unobstructed mesopores, validating their anchoring within the internal structure of the support.
View Article and Find Full Text PDFChemistry
January 2025
Nanjing University of Aeronautics and Astronautics, School of Materials Science and Engineering, 29 Yudao St., 210016, Nanjing, CHINA.
As a potential alternative to next-generation LIBs, carbonous materials have garnered significant attention as anode materials for potassium-ion batteries due to their low cost and environmental friendliness. However, carbonaceous materials cannot fulfill the demand of anode for PIBs, due to volume expansion and poor stability during charging/discharging process. It is well-known that N doping can provide active sites for K-storage, and expand the layer distance between graphite layers.
View Article and Find Full Text PDFRev Sci Instrum
January 2025
Department Spins in Energy Conversion and Quantum Information Science (ASPIN), Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Hahn-Meitner-Platz 1, 14109 Berlin, Germany.
Confocal microscopy is an invaluable tool for studying fluorescent materials and finds a wide application in biology and in quantum sensing. Usually, these experiments are performed under ambient conditions, but many materials are air sensitive (for example, black phosphorus) and degrade quickly under the strong laser irradiance. Here, we present a glovebox-integrated confocal microscope designed for nitrogen-vacancy (NV) center-based nano-scale sensing and NMR spectroscopy in an inert gas atmosphere.
View Article and Find Full Text PDFNat Commun
January 2025
Department of Chemical and Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, 117585, Singapore, Singapore.
Photocatalytic conversion has emerged as a promising strategy for harnessing renewable solar energy in the valorization of plastic waste. However, research on the photocatalytic transformation of plastics into valuable nitrogen-containing chemicals remains limited. In this study, we present a visible-light-driven pathway for the conversion of polylactic acid (PLA) into alanine under mild conditions.
View Article and Find Full Text PDFSci Rep
January 2025
Key Laboratory of Micro/nano Devices and Systems, Ministry of Education, North University of China, Taiyuan, 030051, China.
As the hyperentanglement of photon systems holds lots of remarkable applications for enhancing channel capacity with less quantum resource, the interconversion of various hyperentangled states warrants in-depth investigation and becomes a vital work for quantum information technologies. Here we realize completely mutual conversions between spatial-polarization hyperentangled Knill-Laflamme-Milburn state and hyperentangled W state for three-photon systems, resorting to hyperparallel quantum control gates and the practical nonlinear interaction of nitrogen-vacancy centers coupled with whispering-gallery-mode microresonators. The hyperparallel quantum gates, i.
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