When a core level is excited by circularly polarized light, the angular momentum of light is transferred to the emitted photoelectron, which can be confirmed by the parallax shift of the forward focusing peak (FFP) direction in a stereograph of atomic arrangement. No angular momentum has been believed to be transferred to normal Auger electrons resulting from the decay process filling core hole after photoelectron ejection. We succeeded in detecting a non-negligible circular dichroism contrast in a normal Auger electron diffraction from a nonmagnetic Cu(001) surface far off from the absorption threshold. Moreover, we detected angular-momentum-polarized Cu L(3)M(4,5)M(4,5) Auger electrons at the L(3) absorption threshold, where the excited core electron is trapped at the conduction band. From the kinetic energy dependence of the Auger electron FFP parallax shift, we found that the angular momentum is transferred to the Auger electron most effectively in the case of the (1)S(0) two-hole creation.
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http://dx.doi.org/10.1103/PhysRevLett.114.015501 | DOI Listing |
Rev Sci Instrum
December 2024
SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA.
We describe the design and performance of a magnetic bottle electron spectrometer (MBES) for high-energy electron spectroscopy. Our design features a 2 m long electron drift tube and electrostatic retardation lens, achieving sub-electronvolt (eV) electron kinetic energy resolution for high energy (several hundred eV) electrons with a close to 4π collection solid angle. A segmented anode electron detector enables the simultaneous collection of photoelectron spectra in high resolution and high collection efficiency modes.
View Article and Find Full Text PDFJ Radiat Res
December 2024
The Center for Peace, Hiroshima University, Higashisenda-machi 1-1-89, Naka-ku, Hiroshima 730-0053, Japan.
Radiobiological studies are ongoing to understand the consequences of internal exposure to neutron-activated radioactive microparticles, which were sprayed over experimental rats and mice. Special attention in these experiments is given to internal irradiation with radioactive microparticles with short-lived neutron-activated radionuclides 31Si (T1/2 = 2.62 h) and 56Mn (T1/2 = 2.
View Article and Find Full Text PDFPhys Chem Chem Phys
December 2024
Jožef Stefan Institute, Jamova cesta 39, 1000 Ljubljana, Slovenia.
We present an theoretical method to calculate the resonant Auger spectrum in the presence of ultrafast dissociation. The method is demonstrated by deriving the L-VV resonant Auger spectrum mediated by the 2pσ* resonance in HCl, where the electronic Auger decay and nuclear dissociation occur on the same time scale. The Auger decay rates are calculated within the one-center approximation and are shown to vary significantly with the inter-nuclear distance.
View Article and Find Full Text PDFACS Appl Mater Interfaces
December 2024
Gordon A. and Mary Cain Department of Chemical Engineering, Louisiana State University, Baton Rouge, Louisiana 70803, United States.
Future processes and materials are needed to enable multichip packages with chip-to-chip (C2C) data rates of 50 GB/s or higher. This presents a fundamental challenge because of the skin effect, which exacerbates signal transmission losses at high frequencies. Our results indicate that smooth copper interconnects with relatively thin cuprous oxides (CuO, Cu) and amine-functional silane adhesion promoters improve interfacial adhesion with epoxy dielectrics by nearly an order of magnitude.
View Article and Find Full Text PDFEJNMMI Radiopharm Chem
December 2024
Life Sciences Division, TRIUMF, 4004 Wesbrook Mall, Vancouver, BC, V6T 2A3, Canada.
Background: Er (t = 10.4 h, E = 47.1 keV (59.
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