Tailoring light-matter coupling in semiconductor and hybrid-plasmonic nanowires.

Rep Prog Phys

Department of Materials Science and Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA.

Published: August 2014

AI Article Synopsis

  • Understanding light-matter interactions is key across various fields, leading to advancements in technologies like lasers, sensors, and modulators.
  • Reducing optical mode volume is essential for increasing light-matter coupling strength, with self-assembled semiconductor and hybrid-plasmonic nanowires offering highly-confined optical modes.
  • Recent progress includes unique spectroscopic techniques that enhance coupling strength in nanowire optical cavities, showcasing significant results like sub-picosecond excited-state lifetimes and improved radiative rates.

Article Abstract

Understanding interactions between light and matter is central to many fields, providing invaluable insights into the nature of matter. In its own right, a greater understanding of light-matter coupling has allowed for the creation of tailored applications, resulting in a variety of devices such as lasers, switches, sensors, modulators, and detectors. Reduction of optical mode volume is crucial to enhancing light-matter coupling strength, and among solid-state systems, self-assembled semiconductor and hybrid-plasmonic nanowires are amenable to creation of highly-confined optical modes. Following development of unique spectroscopic techniques designed for the nanowire morphology, carefully engineered semiconductor nanowire cavities have recently been tailored to enhance light-matter coupling strength in a manner previously seen in optical microcavities. Much smaller mode volumes in tailored hybrid-plasmonic nanowires have recently allowed for similar breakthroughs, resulting in sub-picosecond excited-state lifetimes and exceptionally high radiative rate enhancement. Here, we review literature on light-matter interactions in semiconductor and hybrid-plasmonic monolithic nanowire optical cavities to highlight recent progress made in tailoring light-matter coupling strengths. Beginning with a discussion of relevant concepts from optical physics, we will discuss how our knowledge of light-matter coupling has evolved with our ability to produce ever-shrinking optical mode volumes, shifting focus from bulk materials to optical microcavities, before moving on to recent results obtained from semiconducting nanowires.

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Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC4859436PMC
http://dx.doi.org/10.1088/0034-4885/77/8/086401DOI Listing

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