Natural, dissolved (238)U-series radionuclides (U, (226)Ra, (222)Rn) and activity ratios (A.R.s: (234)U/(238)U; (228)Ra/(226)Ra) in Continental Intercalaire (CI) groundwaters and limited samples from the overlying Complexe Terminal (CT) aquifers of Algeria and Tunisia are discussed alongside core measurements for U/Th (and K) in the contexts of radiological water quality, geochemical controls in the aquifer, and water residence times. A redox barrier is characterised downgradient in the Algerian CI for which a trend of increasing (234)U/(238)U A.R.s with decreasing U-contents due to recoil-dominated (234)U solution under reducing conditions allows residence time modelling ∼500 ka for the highest enhanced A.R. = 3.17. Geochemical modelling therefore identifies waters towards the centre of the Grand Erg Oriental basin as palaeowaters in line with reported (14)C and (36)Cl ages. A similar (234)U/(238)U trend is evidenced in a few of the Tunisian CI waters. The paleoage status of these waters is affirmed by both noble gas recharge temperatures and simple modelling of dissolved, radiogenic (4)He-contents both for sampled Algerian and Tunisian CI and CT waters. For the regions studied these waters therefore should be regarded as "fossil" waters and treated effectively as a non-renewable resource.
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