A laser-boosted relativistic solid-density paraboloidal foil is known to efficiently reflect and focus a counterpropagating laser pulse. Here we show that in the case of an ultrarelativistic counterpropagating pulse, a high-energy and ultrahigh-intensity reflected pulse can be more effectively generated by a relatively slow and heavy foil than by a fast and light one. This counterintuitive result is explained with the larger reflectivity of a heavy foil, which compensates for its lower relativistic Doppler factor. Moreover, since the counterpropagating pulse is ultrarelativistic, the foil is abruptly dispersed and only the first few cycles of the counterpropagating pulse are reflected. Our multidimensional particle-in-cell simulations show that even few-cycle counterpropagating laser pulses can be further shortened (both temporally and in the number of laser cycles) with pulse amplification. A single few-cycle, multipetawatt laser pulse with several joules of energy and with a peak intensity exceeding 10(23) W/cm(2) can be generated already employing next-generation high-power laser systems. In addition, the carrier-envelope phase of the generated few-cycle pulse can be tuned provided that the carrier-envelope phase of the initial counterpropagating pulse is controlled.
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http://dx.doi.org/10.1103/PhysRevLett.113.025005 | DOI Listing |
Nanophotonics
April 2024
TUM School of Computation, Information and Technology, Technical University of Munich (TUM), D-85748 Garching, Germany.
In research and engineering, short laser pulses are fundamental for metrology and communication. The generation of pulses by passive mode-locking is especially desirable due to the compact setup dimensions, without the need for active modulation requiring dedicated external circuitry. However, well-established models do not cover regular self-pulsing in gain media that recover faster than the cavity round trip time.
View Article and Find Full Text PDFVelocity-map imaging (VMI) is a key tool for studying outgoing electrons or ions following optical strong-field interactions of atoms and molecules and provides good momentum resolution even if the source volume of the fragments extends along a laser beam path. Here, we demonstrate within an enhancement cavity how, independently of the focal Rayleigh length, counter-propagating pulses longitudinally compress the ionization volume down to few tens of micrometers. We observe nonlinear above-threshold ionization (ATI) processes confined to the spatial overlap of femtosecond pulses, whereas the shortened ionization volume makes an electrostatic lens unnecessary for VMI.
View Article and Find Full Text PDFUltrafast laser pulse filamentation in the air can be used for remote sensing by exciting a characteristic optical emission, which is usually referred to as filamentation-induced breakdown spectroscopy. In environments that impede light propagation, such as fog, haze, or clouds, scattering makes it challenging to propagate laser beams and retrieve generated optical signatures. We demonstrate the effectiveness of laser filamentation for simultaneously clearing the path for intense femtosecond pulse propagation in a highly scattering medium, generation of luminous plasma on a solid target, and counter-propagation of a characteristic spectroscopic signal over a cleared channel along the filament path.
View Article and Find Full Text PDFPhys Rev E
June 2024
State Key Laboratory of Nuclear Physics and Technology, and Key Laboratory of HEDP of the Ministry of Education, CAPT, School of Physics, Peking University, Beijing 100871, China.
Collision between relativistic electron sheets and counterpropagating laser pulses is recognized as a promising way to produce intense attosecond x rays through coherent Thomson backscattering (TBS). In a double-layer scheme, the electrons in an ultrathin solid foil are first pushed out by an intense laser driver and then interact with the laser reflected off a second foil to form a high-density relativistic electron sheet with vanishing transverse momentum. However, the repulsion between these concentrated electrons can increase the thickness of the layer, reducing both its density and subsequently the coherent TBS.
View Article and Find Full Text PDFAnal Chem
July 2024
Department of Chemistry, University of Kansas, Lawrence, Kansas 66045, United States.
Applications involving two-photon activation, including two-photon fluorescence imaging, photodynamic therapy, and 3D data storage, require precise knowledge of the two-photon absorption (2PA) spectra of target chromophores. Broadband pump-probe spectroscopy using femtosecond laser pulses provides wavelength-dependent 2PA spectra with absolute cross sections, but the measurements are sometimes complicated by cross-phase modulation effects and dispersion of the broadband probe. Here, we introduce a single-shot approach that eliminates artifacts from cross-phase modulation and enables more rapid measurements by avoiding the need to scan the time delay between the pump and the probe pulses.
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