The Gamow-Teller strength in the β(+) direction to (46)Sc was extracted via the (46)Ti(t,(3)He + γ) reaction at 115 MeV/u. The γ-ray coincidences served to precisely measure the very weak Gamow-Teller transition to a final state at 991 keV. Although this transition is weak, it is crucial for accurately estimating electron-capture rates in astrophysical scenarios with relatively low stellar densities and temperatures, such as presupernova stellar evolution. Shell-model calculations with different effective interactions in the pf shell-model space do not reproduce the experimental Gamow-Teller strengths, which is likely due to sd-shell admixtures. Calculations in the quasiparticle random phase approximation that are often used in astrophysical simulations also fail to reproduce the experimental Gamow-Teller strength distribution, leading to strongly overestimated electron-capture rates. Because reliable theoretical predictions of Gamow-Teller strengths are important for providing astrophysical electron-capture reaction rates for a broad set of nuclei in the lower pf shell, we conclude that further theoretical improvements are required to match astrophysical needs.
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http://dx.doi.org/10.1103/PhysRevLett.112.252501 | DOI Listing |
Phys Rev Lett
December 2024
Department of Physics, Kyungpook National University, Daegu 41566, Republic of Korea.
We give for the first time theoretical estimates of unknown rare electron-capture (EC) decay branchings of ^{44}Ti, ^{57}Co, and ^{139}Ce, relevant for searches of (exotic) dark-matter particles. The nuclear-structure calculations have been done exploiting the nuclear shell model with well-established Hamiltonians and an advanced theory of β decay. In the absence of experimental measurements of these rare branches, these estimates are of utmost importance for terrestrial searches of dark-matter particles, such as axionic dark matter in the form of axionlike particles, anapole dark matter, and dark photons in nuclear transitions.
View Article and Find Full Text PDFHeliyon
December 2024
Aix Marseille Univ, LCE, Marseille, France.
Bromobenzoquinones and 2,4,6-tribromophenol belong to disinfection or chlorination by-products than can be formed in bromide-rich waters during chlorination or chloramination. Due to their high toxicities, sensitive and cost-effective analytical methods are necessary to detect and quantify them in various environmental matrices. A determination method of 2,5-dibromo-1,4-benzoquinone, 2,6-dibromo-3,5-dimethyl-1,4-benzoquinone, 2,6-dibromo-3-chloro-5-methyl-1,4-benzoquinone, 2,3,5,6-tetrabromo-1,4-benzoquinone and, 2,4,6-tribromophenol was developed using solid-phase extraction and electron capture detector-gas chromatography separation and detection (SPE-GC-ECD).
View Article and Find Full Text PDFAppl Radiat Isot
September 2024
Institut für Physik, Johannes Gutenberg Universität Mainz, Staudingerweg 7, D-55128, Mainz, Germany.
Terbium-157 was radiochemically extracted from an irradiated tantalum target. Since the resulting material contained a significant impurity of Tb, Tb was isotopically purified using laser resonance ionization at the RISIKO mass separator in Mainz and then implanted on an aluminum (Al) foil. The implanted Tb was measured by two different calibrated gamma-ray spectrometers to determine photon emission rates.
View Article and Find Full Text PDFSci Total Environ
November 2023
Department of Chemistry, Chemical Biological Centre (KBC), Umeå University, Linnaeus väg 6, 901 87, Umeå, Sweden.
A time-trend study was carried out for two important Baltic Sea species, blue mussel (1994-2017, 11 samples) and eelpout (1994-2017, 11 samples), to track the changes in levels of regulated persistent organic pollutants (POPs) and show potential increases in the levels of the contaminants of emerging concern (CECs). It was carried out utilizing gas chromatography-high-resolution mass spectrometry (GC-HRMS) based non-target screening (NTS). Data were acquired in two modes - electron ionization (EI) and electron capture negative ion chemical ionization (ECNI) - to widen the contaminant coverage, and treated using a fast semi-automated NTS data processing workflow.
View Article and Find Full Text PDFSensors (Basel)
June 2023
National Institute of Materials Physics, Atomistilor 405A, 077125 Magurele, Ilfov, Romania.
The acceptor removal process is the most detrimental effect encountered in irradiated boron-doped silicon. This process is caused by a radiation-induced boron-containing donor (BCD) defect with bistable properties that are reflected in the electrical measurements performed in usual ambient laboratory conditions. In this work, the electronic properties of the BCD defect in its two different configurations (A and B) and the kinetics behind transformations are determined from the variations in the capacitance-voltage characteristics in the 243-308 K temperature range.
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