Penning ionization initiates the evolution of a dense molecular Rydberg gas to plasma. This process selects for pairs of excited molecules separated by a distance of two Rydberg orbital diameters or less. The deactivated Penning partners predissociate, depleting the leading edge of the distribution of nearest-neighbor distances. For certain density and orbital radii, this sequence of events can form a plasma in which large distances separate a disproportionate fraction of the ions. Experimental results and model calculations suggest that the reduced potential energy of this Penning lattice significantly affects the development of strong coupling in an ultracold plasma.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1103/PhysRevLett.112.075001 | DOI Listing |
Molecules
October 2024
Institute of Theoretical and Computational Chemistry, Key Laboratory of Mesoscopic Chemistry, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210023, China.
Three-body recombination reactions, in which two particles form a bound state while a third one bounces off after the collision, play significant roles in many fields, such as cold and ultracold chemistry, astrochemistry, atmospheric physics, and plasma physics. In this work, the dynamics of the recombination reaction for the N system over a wide temperature range (5000-20,000 K) are investigated in detail using the quasi-classical trajectory (QCT) method based on recently developed full-dimensional potential energy surfaces. The recombination products are N() + N() in the 1″ state, N() + N() in the 2″ state, and N() + N() in both the 1″ and 2″ states.
View Article and Find Full Text PDFJ Chem Phys
October 2024
Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 730000, China.
Inelastic n-changing collisions play an important role in the evolution of Rydberg atoms into ultracold plasmas. However, for the initially intermediate n (n ∼ 40) Rydberg states, these collisions can hardly be observed due to the low electron temperature in ultracold plasmas. In this work, we designed an experimental scheme to facilitate collisions between free electrons at 1.
View Article and Find Full Text PDFPhys Rev E
August 2024
Joint Institute for High Temperatures, Russian Academy of Sciences, Izhorskaya Street 13, 125412 Moscow, Russia.
In this Reply, we respond to the Comment by Schlitters et al. on our recent work [Phys. Rev.
View Article and Find Full Text PDFPhys Rev E
August 2024
Department of Physics and Astronomy, Brigham Young University, Provo, Utah 84602, USA.
Bronin et al. [Phys. Rev.
View Article and Find Full Text PDFPhys Rev E
July 2024
Department of Physics and Institute for Fundamental Science, University of Oregon, Eugene, Oregon 97403, USA.
Motivated by a number of realizations of long-range interacting systems, including ultracold atomic and molecular gases, we study a neutral plasma with power-law interactions longer ranged than Coulombic. We find that beyond a crossover length, such interactions are universally screened down to a standard Coulomb form in all spatial dimensions. This implies, counterintuitively, that in two dimensions and below, such a "super-Coulombic" gas is asymptotically Coulombically confining at low temperatures.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!