We report measurements of electrical transport through single CdSe/CdS core/shell colloidal quantum dots (cQDs) connected to source and drain contacts. We observe telegraphic switching noise showing few plateaus at room temperature. We model and interpret these results as charge trapping of individual trap states, and therefore we resolve individual charge defects in these high-quality low-strain cQDs. The small number of observed defects quantitatively validates the passivation method based on thick CdS shells nearly lattice-matched to CdSe cores first developed to suppress photoluminescence blinking. Finally, we introduce a figure of merit useful to efficiently distinguish telegraphic noise from noise with a Gaussian distribution.
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http://dx.doi.org/10.1021/nl404247e | DOI Listing |
ACS Nano
January 2025
Department of Physics, Indian Institute of Science, Bangalore 560012, India.
The low-frequency resistance fluctuations, or noise, in electrical resistance not only set a performance benchmark in devices but also form a sensitive tool to probe nontrivial electronic phases and band structures in solids. Here, we report the measurement of such noise in the electrical resistance in twisted bilayer graphene (tBLG), where the layers are misoriented close to the magic angle (θ ∼ 1°). At high temperatures ( ≳ 60-70 K), the power spectral density (PSD) of the fluctuation inside the low-energy moiré bands is predominantly ∝1/, where is the frequency, being generally lowest close to the magic angle, and can be well-explained within the conventional McWhorter model of the '1/ noise' with trap-assisted density-mobility fluctuations.
View Article and Find Full Text PDFPhys Rev E
November 2024
School of Physics, Korea Institute for Advanced Study, Seoul 02455, Republic of Korea.
Stochastic resetting has recently emerged as an efficient target-searching strategy in various physical and biological systems. The efficiency of this strategy depends on the type of environmental noise, whether it is thermal or telegraphic (active). While the impact of each noise type on a search process has been investigated separately, their combined effects have not been explored.
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November 2024
Empa, nanotech@surfaces Laboratory, Dübendorf CH-8600, Switzerland.
Understanding single molecular switches is a crucial step in designing and optimizing molecular electronic devices with highly nonlinear functionalities, e.g., gate voltage-dependent current switching.
View Article and Find Full Text PDFPhys Rev E
May 2024
LPTMS, CNRS, Université Paris-Sud, Université Paris-Saclay, 91405 Orsay, France.
The study of diffusion with preferential returns to places visited in the past has attracted increased attention in recent years. In these highly non-Markov processes, a standard diffusive particle intermittently resets at a given rate to previously visited positions. At each reset, a position to be revisited is randomly chosen with a probability proportional to the accumulated amount of time spent by the particle at that position.
View Article and Find Full Text PDFPhys Rev E
November 2022
Department of Biomedical Engineering, Ben-Gurion University of the Negev, Marcus Family Campus Be'er Sheva, 8410501, Israel.
We study the full nonequilibrium steady-state distribution P_{st}(X) of the position X of a damped particle confined in a harmonic trapping potential and experiencing active noise whose correlation time τ_{c} is assumed to be very short. Typical fluctuations of X are governed by a Boltzmann distribution with an effective temperature that is found by approximating the noise as white Gaussian thermal noise. However, large deviations of X are described by a non-Boltzmann steady-state distribution.
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