Exciton liquid in coupled quantum wells.

Science

Department of Condensed Matter Physics, Weizmann Institute of Science, Rehovot, Israel.

Published: January 2014

Excitons in semiconductors may form correlated phases at low temperatures. We report the observation of an exciton liquid in gallium arsenide/aluminum gallium arsenide-coupled quantum wells. Above a critical density and below a critical temperature, the photogenerated electrons and holes separate into two phases: an electron-hole plasma and an exciton liquid, with a clear sharp boundary between them. The two phases are characterized by distinct photoluminescence spectra and by different electrical conductance. The liquid phase is formed by the repulsive interaction between the dipolar excitons and exhibits a short-range order, which is manifested in the photoluminescence line shape.

Download full-text PDF

Source
http://dx.doi.org/10.1126/science.1243409DOI Listing

Publication Analysis

Top Keywords

exciton liquid
12
quantum wells
8
liquid coupled
4
coupled quantum
4
wells excitons
4
excitons semiconductors
4
semiconductors form
4
form correlated
4
correlated phases
4
phases low
4

Similar Publications

Molten Sn solvent expands liquid metal catalysis.

Nat Commun

January 2025

School of Chemical and Biomolecular Engineering, The University of Sydney, Sydney, Australia.

Regulating favorable assemblies of metallic atoms in the liquid state provides promise for catalyzing various chemical reactions. Expanding the selection of metallic solvents, especially those with unique properties and low cost, enables access to distinctive fluidic atomic structures on the surface of liquid alloys and offers economic feasibility. Here, Sn solvent, as a low-cost commodity, supports unique atomic assemblies at the interface of molten SnInCu, which are highly selective for H synthesis from hydrocarbons.

View Article and Find Full Text PDF

Schlieren texture and topography induced confinement in an organic exciton-polariton laser.

Nat Commun

January 2025

Humboldt Centre for Nano- and Biophotonics, Institute for Light and Matter, Department of Chemistry and Biochemistry, University of Cologne, Köln, Germany.

Non-linearities in organic exciton-polariton microcavities represent an attractive platform for quantum devices. However, progress in this area hinges on the development of material platforms for high-performance polariton lasing, scalable and sustainable fabrication, and ultimately strategies for electrical pumping. Here, we show how introducing Schlieren texturing and a rough intra-cavity topography in a liquid crystalline conjugated polymer enables strong in-plane confinement of polaritons and drastic enhancement of the lasing properties.

View Article and Find Full Text PDF

The ability to convert light to higher energies through triplet-triplet annihilation upconversion (TTA-UC) is attractive for a range of applications including solar energy harvesting, bioimaging and anti-counterfeiting. Practical applications require integration of the TTA-UC chromophores within a suitable host, which leads to a compromise between the high upconversion efficiencies achievable in liquids and the durability of solids. Herein, we present a series of methacrylate copolymers as TTA-UC hosts, in which the glass transition temperature ( ), and hence upconversion efficiency can be tuned by varying the co-monomer ratios (-hexyl methacrylate (HMA) and 2,2,2-trifluoroethyl methacrylate (TFEMA)).

View Article and Find Full Text PDF

Leveraging Multivalent Assembly towards High-Temperature Liquid-Phase Phosphorescence.

Angew Chem Int Ed Engl

January 2025

Key Laboratory of Advanced Marine Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, 315201, P. R. China.

High-temperature phosphorescence (HTP) materials have attracted considerable attention owing to their expanded application prospects, whereas they still suffer from severe deactivation in polar media, limiting their reliability and utility. Here, we present an efficient multivalent assembly strategy to achieve high-temperature liquid-phase phosphorescence (HTLP). The supramolecular assembly of multivalent modules leads to extremely robust hydrogen-bonding networks, which firmly immobilize the organic phosphors and protect triplet excitons from annihilation in high-temperature polar media, resulting in excellent HTLP emission.

View Article and Find Full Text PDF

ConspectusThe emergence of two-dimensional (2D) materials, such as graphene, transition-metal dichalcogenides (TMDs), and hexagonal boron nitride (h-BN), has sparked significant interest due to their unique physicochemical, optical, electrical, and mechanical properties. Furthermore, their atomically thin nature enables mechanical flexibility, high sensitivity, and simple integration onto flexible substrates, such as paper and plastic.The surface chemistry of a nanomaterial determines many of its properties, such as its chemical and catalytic activity.

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!