Recent analysis of satellite data obtained during the 9 October 2012 geomagnetic storm identified the development of peaks in electron phase space density, which are compelling evidence for local electron acceleration in the heart of the outer radiation belt, but are inconsistent with acceleration by inward radial diffusive transport. However, the precise physical mechanism responsible for the acceleration on 9 October was not identified. Previous modelling has indicated that a magnetospheric electromagnetic emission known as chorus could be a potential candidate for local electron acceleration, but a definitive resolution of the importance of chorus for radiation-belt acceleration was not possible because of limitations in the energy range and resolution of previous electron observations and the lack of a dynamic global wave model. Here we report high-resolution electron observations obtained during the 9 October storm and demonstrate, using a two-dimensional simulation performed with a recently developed time-varying data-driven model, that chorus scattering explains the temporal evolution of both the energy and angular distribution of the observed relativistic electron flux increase. Our detailed modelling demonstrates the remarkable efficiency of wave acceleration in the Earth's outer radiation belt, and the results presented have potential application to Jupiter, Saturn and other magnetized astrophysical objects.
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JACS Au
January 2025
CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology of China, CAS, Beijing 100190, China.
DNA nanostructures present new opportunities as Nanotags for electron microscopy (EM) imaging, leveraging their high programmability, unique shapes, biomolecule conjugation capability, and stability compatible with standard cryogenic sample preparation protocols. This perspective highlights the potential of DNA Nanotags to enable high-throughput multiplexed EM analysis and facilitate particle identification for cryogenic electron tomography (cryo-ET). Meanwhile, applying Nanotags in live-cell environments requires the efficient cellular uptake of intact structures and successful cytosolic migration.
View Article and Find Full Text PDFJ Phys Chem Lett
January 2025
Institute for Sustainable Energy/Department of Chemistry, College of Sciences, Shanghai University, Shanghai 200444, China.
The migration of Zn ions is significantly more challenging compared to that of Li ions within the same crystalline framework, leading to poor rate performance of zinc-ion batteries (ZIBs). Compared to Li, the slower migration rate of Zn is vaguely attributed to the stronger electrostatic interaction induced by Zn. Herein, the rule of how the size of the migration channel and electrostatic interaction affect Zn and Li migration in α-VO has been systematically investigated by first-principle calculations.
View Article and Find Full Text PDFEnviron Pollut
January 2025
Institute of Environmental and Occupational Health Sciences, National Taiwan University, Taiwan. Electronic address:
Despite polychlorinated biphenyls (PCBs) have been banned in Taiwan for two decades, epidemiological studies indicated that prenatal PCBs exposure may still affect newborns and their birth outcomes. The study aimed to investigate the association between PCB concentrations in umbilical cord blood and infants' birth outcomes and neurodevelopment. We recruited 100 pairs of mothers and infants, residing in Changhua and Yunlin countries in Taiwan from 2014-2016.
View Article and Find Full Text PDFACS Nano
January 2025
Department of Chemistry, University of California Berkeley, Berkeley, California 94720, United States.
Understanding charge transport in semiconductor quantum dot (QD) assemblies is important for developing the next generation of solar cells and light-harvesting devices based on QD technology. One of the key factors that governs the transport in such systems is related to the hybridization between the QDs. Recent experiments have successfully synthesized QD molecules, arrays, and assemblies by directly fusing the QDs, with enhanced hybridization leading to high carrier mobilities and coherent band-like electronic transport.
View Article and Find Full Text PDFInorg Chem
January 2025
Institute of Inorganic Chemistry, RWTH Aachen University, 52056 Aachen, Germany.
The ternary transition-metal cyanamide MnCr(NCN) was synthesized by a solid-state metathesis reaction between MnCl, CrCl, and ZnNCN. Powder X-ray diffraction reveals that MnCr(NCN) adopts an orthorhombic [NiAs]-derived structure with symmetry, featuring a hexagonally close-packed array of NCN with metal cations in 3/4 of the octahedral interstitial holes. The question of cation order was addressed via the combinatorial use of X-ray powder diffraction, neutron powder diffraction, electron diffraction, and HAADF-STEM measurements.
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