We report on the tailoring of quantum dot (QD) emission efficiency by localized surface plasmon polaritons in self-organized mesoscopic rings. Ag nanoparticles (NPs) with CdSe QDs embedded in a polymeric matrix are spatially organised in mesoscopic rings and coupled in a tuneable fashion by breath figure formation. The mean distance between NPs and QDs and consequently the intensity of QD photoluminescence, which is enhanced by the coupling of surface plasmons and excitons, are tuned by acting on the NP concentration.
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http://dx.doi.org/10.1039/c3nr04708c | DOI Listing |
Water Sci Technol
June 2024
School of Mechanical Engineering, University of Science and Technology Beijing, Beijing 100083, China; School of Engineering and Applied Sciences, Harvard University, Cambridge, MA 02138, USA E-mail:
In a fluid environment, biofilms usually form and grow into streamers attached to solid surfaces. Existing research on single streamers studied their formation and failure modes. In the experiment on biofilm growth in a microfluidic channel, we found that rings composed of bacteria and an extracellular matrix are important elements on a mesoscopic scale.
View Article and Find Full Text PDFOrg Lett
May 2024
Key Laboratory of Mesoscopic Chemistry of MOE, Jiangsu Key Laboratory of Advanced Organic Materials, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210023, China.
Glycoluril-expanded pillararenes composed of glycoluril and dialkoxybenzene units, namely, pillarurilarenes (), were synthesized through a fragment coupling macrocyclization strategy. Partial replacement of dialkoxybenzene with glycoluril endows with polarized equatorial methine protons for derivatization or CH-anion binding. Crystal structures of pillar[2]uril[4]arene and pillar[1]uril[4]arene containing two glycoluril units and one glycoluril unit, respectively, indicated the inward orientation of the glycoluril unit, as also suggested by H nuclear magnetic resonance and density functional theory calculation.
View Article and Find Full Text PDFPhys Rev Lett
March 2024
Department of Physics, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801-3080, USA.
We introduce feedback-measurement technologies to achieve flexible control of Weyl points and conduct the first experimental demonstration of Weyl type I-II transition in mechanical systems. We demonstrate that non-Hermiticity can expand the Fermi arc surface states from connecting Weyl points to Weyl rings, and lead to a localization transition of edge states influenced by the interplay between band topology and the non-Hermitian skin effect. Our findings offer valuable insights into the design and manipulation of Weyl points in mechanical systems, providing a promising avenue for manipulating topological modes in non-Hermitian systems.
View Article and Find Full Text PDFFront Optoelectron
March 2024
State Key Laboratory for Mesoscopic Physics and Department of Physics, Collaborative Innovation Center of Quantum Matter and Frontiers Science Center for Nano-Optoelectronics, Beijing Academy of Quantum Information Sciences, Peking University, Beijing, 100871, China.
Modulation of topological phase transition has been pursued by researchers in both condensed matter and optics research fields, and has been realized in Euclidean systems, such as topological photonic crystals, topological metamaterials, and coupled resonator arrays. However, the spin-controlled topological phase transition in non-Euclidean space has not yet been explored. Here, we propose a non-Euclidean configuration based on Möbius rings, and we demonstrate the spin-controlled transition between the topological edge state and the bulk state.
View Article and Find Full Text PDFNat Phys
October 2023
Institute of Science and Technology Austria (ISTA), Klosterneuburg, Austria.
The emergence of large-scale order in self-organized systems relies on local interactions between individual components. During bacterial cell division, FtsZ-a prokaryotic homologue of the eukaryotic protein tubulin-polymerizes into treadmilling filaments that further organize into a cytoskeletal ring. In vitro, FtsZ filaments can form dynamic chiral assemblies.
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