The thickness change of a film is measured optically using self-interference of a single laser beam incident at the edge of the film. Theory suggests that when a half-plane phase shift is applied to a Gaussian laser beam, interference fringes appear in the near and far field, in which position varies with the amount of phase shift. By measuring fringe pattern displacement, we demonstrate detection of thickness changes in chitosan films induced by temperature rises of a few degrees centigrade. With a laser at 543 nm, the minimum detectable thickness change is 0.8 nm in ideal conditions (quarter wave films), corresponding with a phase shift of 0.02 rad, and the minimum detectable film thickness is ∼30 nm. Potential use for surface temperature measurements is discussed.
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http://dx.doi.org/10.1364/AO.52.005979 | DOI Listing |
Anal Chem
January 2025
State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Wuhan 430074, PR China.
The elemental imaging of laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS) provides spatial information on elements and therefore can further investigate the growth or evolution processes of an analyte. However, the accurate determination of spatial information is limited by the decoupling between the elemental distribution and mass spectrometry signals. This phenomenon, which is more distinct when high-diffusion ablation cells are used, arises from the overlap of ablation and the transport dispersion of aerosols.
View Article and Find Full Text PDFStruct Dyn
January 2025
Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607 Hamburg, Germany.
Sub-ångström spatial resolution of electron density coupled with sub-femtosecond to few-femtosecond temporal resolution is required to directly observe the dynamics of the electronic structure of a molecule after photoinitiation or some other ultrafast perturbation, such as by soft X-rays. Meeting this challenge, pushing the field of quantum crystallography to attosecond timescales, would bring insights into how the electronic and nuclear degrees of freedom couple, enable the study of quantum coherences involved in molecular dynamics, and ultimately enable these dynamics to be controlled. Here, we propose to reach this realm by employing convergent-beam x-ray crystallography with high-power attosecond pulses from a hard-x-ray free-electron laser.
View Article and Find Full Text PDFBiomed Opt Express
January 2025
School of Optometry, Indiana University, Bloomington, IN, USA.
To measure the influence of ganglion cell layer (GCL) thickness on the changes in size and red blood cell (RBC) flow in small retinal vessels evoked by full-field flicker. We used a dual-beam adaptive optics scanning laser ophthalmoscope to image 11 healthy young controls in two retinal areas with significantly different GCL thicknesses. All capillaries and arterioles of the superficial vascular plexus were responsive to the flicker stimulation.
View Article and Find Full Text PDFA novel, to the best of our knowledge, approach for the modal decomposition of a fiber laser beam is demonstrated using a spatial mode multiplexer. Since the modal decomposition is carried out optically, this approach is able to obtain the modal content at speeds up to the GHz level. In order to demonstrate such performance, we have applied this approach to the modal analysis of a -switched pulse generated in a multimode fiber with alternating intra-pulse mode content.
View Article and Find Full Text PDFWe demonstrate experimentally an efficient terahertz emitter that consists of a 20 µm thick layer of LiNbO clamped between a fused silica substrate and a Si semicone. A focused laser beam from an ultrafast optical oscillator propagates in the LiNbO layer and emits a Cherenkov cone of terahertz radiation to the Si semicone. The radiation is totally internally reflected by the semicone's convex surface and escapes the semicone through its base as a collimated beam.
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