Correlation between Raman sum and optical conductivity sum in La(2-x)Sr(x)CuO4.

J Phys Condens Matter

Department of Physics, Arts and Science, Petroleum Institute, PO Box 2533, Abu Dhabi, UAE. Department of Physics, Faculty of Science, Nagoya University, Furo-cho, Chikusa-ku, Nagoya 464-8602, Japan.

Published: October 2013

AI Article Synopsis

  • In strongly correlated electron systems, the single-particle spectral function shows a transition to coherent peaks and incoherent humps over 1 eV, with the incoherent parts losing symmetry.
  • The B1g and B2g Raman spectra in underdoped La(2-x)Sr(x)CuO4 become identical above 2000 cm(-1) when certain scattering effects are removed, indicating a connection to optical conductivity.
  • The mid-infrared absorption spectrum reveals a hump between 1000 and 4000 cm(-1), linked to magnetic excitations from hole hopping in antiferromagnetic spin stripes, reflecting the behavior of incoherent electronic states at low carrier densities.

Article Abstract

In a strongly correlated electron system, the single-particle spectral function changes into a coherent peak and incoherent humps which extend over 1 eV. The incoherent parts lose the symmetry and k dependence, so that the Raman spectra with different symmetries become identical and they are expressed by the optical conductivity. We found that the B1g and B2g spectra in La(2-x)Sr(x)CuO4 become identical above 2000 cm(-1) in the underdoped phase, if Fleury-Loudon type B1g two-magnon scattering is removed. The first Raman susceptibility moment correlates with the generalized optical conductivity moment. The good correlation arises from the incoherent states of a hump from 1000 to 4000 cm(-1). The hump is the only structure of the incoherent electronic states in the mid-infrared absorption spectra below 1.4 eV at low carrier densities. The energy is twice the separated dispersion segments of the spin wave in the k(perpendicular) stripe direction. The incoherent state is formed by the magnetic excitations created by the hole hopping in the antiferromagnetic spin stripes in the real space picture.

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Source
http://dx.doi.org/10.1088/0953-8984/25/41/415701DOI Listing

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