We present a theoretical study of high-order harmonic generation (HHG) and propagation driven by an infrared field carrying orbital angular momentum (OAM). Our calculations unveil the following relevant phenomena: extreme-ultraviolet harmonic vortices are generated and survive to the propagation effects, vortices transport high-OAM multiples of the corresponding OAM of the driving field and, finally, the different harmonic vortices are emitted with similar divergence. We also show the possibility of combining OAM and HHG phase locking to produce attosecond pulses with helical pulse structure.
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http://dx.doi.org/10.1103/PhysRevLett.111.083602 | DOI Listing |
J Phys Chem A
January 2025
School of Physics and Electronic Technology, Liaoning Normoal University, Dalian 116081, People's Republic of China.
Photolysis of energetic materials offers safer and more controllable advantages compared to traditional ignition methods. Tracking the group and electron dynamics during the photolysis of energetic materials is currently a hot and challenging topic. In this work, we used a time-dependent density functional theory (TDDFT) to study the high-order Harmonic generation (HHG) dynamics induced by strong laser interaction with an isolated CHNO molecule with varying C-N bond lengths.
View Article and Find Full Text PDFNat Commun
December 2024
Wuhan Institute of Physics and Mathematics, Innovation Academy for Precision Measurement Science and Technology, Chinese Academy of Sciences, Wuhan, 430071, China.
Electron diffraction spectroscopy is a fundamental tool for investigating quasicrystal structures, which unveils the quasiperiodic long-range order. Nevertheless, it falls short in effectively distinguishing separate local isomorphism classes. This is a long outstanding problem.
View Article and Find Full Text PDFBrain Struct Funct
December 2024
Sensory and Motor Systems Research Group, Korea Brain Research Institute, Daegu, South Korea.
Vocal learners, including humans and songbirds, acquire their complex vocalizations by accurately memorizing and imitating the vocal patterns of other individuals. In songbirds, the caudomedial nidopallium (NCM), considered the secondary auditory region, has been suggested to play a critical role in memorizing and recognizing the songs of tutors. However, the mechanisms by which NCM neurons encode the acoustic information of tutor song are not yet fully understood.
View Article and Find Full Text PDFNanophotonics
August 2024
Friedrich-Schiller University Jena, Jena, Germany.
High-order harmonic generation (HHG) in solids opens new frontiers in ultrafast spectroscopy of carrier and field dynamics in condensed matter, picometer resolution structural lattice characterization and designing compact platforms for attosecond pulse sources. Nanoscale structuring of solid surfaces provides a powerful tool for controlling the spatial characteristics and efficiency of the harmonic emission. Here we study HHG in a prototypical phase-change material GeSbTe (GST).
View Article and Find Full Text PDFNanophotonics
August 2024
School of Physics and Technology and Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education, Wuhan University, Wuhan 430072, China.
High-order wave mixing in solid-state platforms gather increasing importance due to the development of advanced lasers and integrated photonic circuit for both classical and quantum information. However, the high-order wave mixing is generally inefficient in solids under weak pump. Here, we observed the presence of phase matching of five-wave mixing (5WM) propagating in a zinc oxide (ZnO) microwire.
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