Complementary theoretical modeling methods are presented for the classical and quantum Heisenberg model to explain the magnetic properties of nanometer-sized magnetic molecules. Excellent quantitative agreement is achieved between our experimental data down to 0.1 K and for fields up to 60 Tesla and our theoretical results for the giant Keplerate species {Mo72Fe30}, by far the largest paramagnetic molecule synthesized to date.

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http://dx.doi.org/10.1002/1439-7641(20010917)2:8/9<517::AID-CPHC517>3.0.CO;2-1DOI Listing

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