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Cyclo-N : a Novel 5/6 Fused Polynitrogen Anion for High Energy Density Materials.
Adv Sci (Weinh)
January 2025
School of Chemistry and Chemical Engineering, Nanjing University of Science and Technology, Nanjing, Jiangsu, 210094, China.
After cyclo-pentazolate anion, a 5/6 fused structure of N is constructed, and four novel nitrogen-rich ionic compounds are assembled on its basis. The results of the quantum calculations revealed an uneven distribution of electrons on cyclo-N , with significant charge density near the N5/N9 atoms and an ADCH charge of -0.425.
View Article and Find Full Text PDFOptimal Neutron Spectrum Database for In-reactor Pu Production.
Adv Sci (Weinh)
January 2025
Science and Technology on Reactor System Design Technology Laboratory, Nuclear Power Institute of China, Chengdu, 610200, China.
Plutonium-238 (Pu) is a scarce heat-source radioisotope used in nuclear batteries, which is produced by in-reactor irradiation of Americium-241 (Am) or Neptunium-237 (Np). Optimizing the neutron spectrum can improve the production efficiency of Pu, but currently, it is still a lack of knowledge about the optimal neutron spectrum for Pu production. Genetic algorithms and burnup algorithms are combined to identify optimal neutron spectra for Pu production under various irradiation times and flux levels, and build an optimal neutron spectrum database, which answers the questions "What is the optimal neutron spectrum for Pu production?" and "What is the maximum efficiency for Pu production" once and for all.
View Article and Find Full Text PDFDual-Induced Directed Deposition Mechanism Based on Anionic Surfactants Enables Long Cycle Aqueous Zinc Ion Batteries.
Small Methods
January 2025
School of Physical Science and Technology, Center for Energy Conversion Materials & Physics (CECMP), Jiangsu Key Laboratory of Thin Films, Soochow University, Suzhou, 215006, China.
Aqueous zinc-ion battery has low cost, and environmental friendliness, emerging as a promising candidate for next-generation battery systems. However, it still suffers from a limited cycling life, caused by dendritic Zn growth and severe side reactions. Recent research highlights that the Zn (002) crystal plane exhibits superior anti-corrosive properties and a horizontal growth pattern.
View Article and Find Full Text PDFElucidating Mesostructural Effects on Thermal Conductivity for Enhanced Insulation Applications.
Small
January 2025
Laboratory of Advanced Materials, Department of Chemistry, Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, State Key Laboratory of Molecular Engineering of Polymers, Collaborative Innovation Center of Chemistry for Energy Materials, Fudan University, Shanghai, 200433, China.
Thermal management is a key link in improving energy utilization and preparing insulation materials with excellent performance is the core technological issue. Complex and irregular pore structures of insulation materials hinder the exploration of structure-property relationships and the further promotion of material performance. Ordered mesoporous silica (OMS) is a kind of porous material with ordered frameworks.
View Article and Find Full Text PDFExploring the progress and trends of immunotherapy for type 1 diabetes: A comprehensive bibliometric analysis spanning nearly two decades.
Obes Rev
January 2025
Department of Endocrinology and Metabolism, The Second Affiliated Hospital, Jiangxi Medical College, Nanchang University, Nanchang, China.
Introduction: Immunotherapy is a crucial treatment for type 1 diabetes (T1D), yet analyses focusing on research priorities and trends in this field are limited. Therefore, this study employs bibliometric methods to systematically explore the current research status of immunotherapy for T1D.
Methods: Based on the Web of Science Core Collection Database, 1573 articles and review articles related to immunotherapy for T1D published from 2004 to 2023 were screened for bibliometric analysis.
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