Conventional semiconductor laser emission relies on stimulated emission of photons, which sets stringent requirements on the minimum amount of energy necessary for its operation. In comparison, exciton-polaritons in strongly coupled quantum well microcavities can undergo stimulated scattering that promises more energy-efficient generation of coherent light by 'polariton lasers'. Polariton laser operation has been demonstrated in optically pumped semiconductor microcavities at temperatures up to room temperature, and such lasers can outperform their weak-coupling counterparts in that they have a lower threshold density. Even though polariton diodes have been realized, electrically pumped polariton laser operation, which is essential for practical applications, has not been achieved until now. Here we present an electrically pumped polariton laser based on a microcavity containing multiple quantum wells. To prove polariton laser emission unambiguously, we apply a magnetic field and probe the hybrid light-matter nature of the polaritons. Our results represent an important step towards the practical implementation of polaritonic light sources and electrically injected condensates, and can be extended to room-temperature operation using wide-bandgap materials.
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http://dx.doi.org/10.1038/nature12036 | DOI Listing |
Sci Adv
January 2025
State Key Laboratory of Extreme Photonics and Instrumentation, College of Optical Science and Engineering, International Research Center for Advanced Photonics, Zhejiang University, Hangzhou 310027, China.
Solution-processed semiconductor lasers are next-generation light sources for large-scale, bio-compatible and integrated photonics. However, overcoming their performance-cost trade-off to rival III-V laser functionalities is a long-standing challenge. Here, we demonstrate room-temperature continuous-wave perovskite polariton lasers exhibiting remarkably low thresholds of ~0.
View Article and Find Full Text PDFMicrosyst Nanoeng
January 2025
National Key Laboratory of Advanced Micro and Nano Manufacture Technology, Beijing, 100871, PR China.
The localized surface plasmon resonance metasurface is a research hotspot in the sensing field since it can enhance the light-matter interaction in the nanoscale, but the wavelength sensitivity is far from comparable with that of prism-coupled surface plasmon polariton (SPP). Herein, we propose and demonstrate an ultrasensitive angular interrogation sensor based on the transverse electric mode surface lattice resonance (SLR) mechanism in an all-metal metasurface. In theory, we derive the sensitivity function in detail and emphasize the refraction effect at the air-solution interface, which influences the SLR position and improves the sensitivity performance greatly in the wide-angle.
View Article and Find Full Text PDFJ Chem Theory Comput
January 2025
Department of Theoretical Physics, University of Debrecen, P.O. Box 400, Debrecen H-4002, Hungary.
The coupling of matter to the quantized electromagnetic field of a plasmonic or optical cavity can be harnessed to modify and control chemical and physical properties of molecules. In optical cavities, a term known as the dipole self-energy (DSE) appears in the Hamiltonian to ensure gauge invariance. The aim of this work is twofold.
View Article and Find Full Text PDFNano Lett
January 2025
State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, 100871 Beijing, China.
Sci Rep
January 2025
MOE Key Laboratory of Laser Life Science, Institute of Laser Life Science, College of Biophotonics, South China Normal University, Guangzhou, 510631, China.
We integrate monolayer TMDCs into silicon-on-insulation (SOI) waveguides and dielectric-loaded surface plasmon polariton (DLSPP) waveguides to enhance nonlinear parameters (γ) of silicon-based waveguides. By optimizing the waveguide geometry, we have achieved significantly improved γ. In MoSe-on-SOI and MoSe-in-DLSPP waveguide with optimized geometry, the maximum γ at the excitonic resonant peak (λ) is 5001.
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