We report generation of 48 fs pulses at a center wavelength of 2070 nm using a degenerate optical parametric oscillator (OPO) synchronously-pumped with a commercially available 36-MHz, femtosecond, mode-locked, Yb-doped fiber laser. The spectral bandwidth of the output is ~137 nm, corresponding to a theoretical, transform-limited pulse width of 33 fs. The threshold of the OPO is less than 10 mW of average pump power. By tuning the cavity length, the output spectrum covers a spectral width of more than 400 nm, limited only by the bandwidth of the cavity mirrors.
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http://dx.doi.org/10.1364/OE.20.027589 | DOI Listing |
A hundred-watt-level peak-power linearly polarized Ho,Pr:GdScO laser with narrow pulses was first realized at ∼3 µm through a combination of theoretical simulation and experiment. This is the narrowest pulse width, and the highest peak power has been achieved in a passively pulsed Ho,Pr co-doped laser to date. We realized a linearly polarized narrow-pulsed laser at ∼3 µm, with a maximum peak power of 185 W and shortest pulse width of 42 ns.
View Article and Find Full Text PDFWe demonstrate a gas-filled multipass cell (MPC) that cleaned the spatial mode of a spatial-filter-free 250 W, 100 kHz, 445 fs driven source based on an Innoslab amplifier and compressed the pulse duration to 41 fs simultaneously. The multipass cell acted as a spatial filter and benefited from its discrete waveguide nature, in which the input beam quality factor M was improved from 1.53 to a near-diffraction-limited value of 1.
View Article and Find Full Text PDFJ Phys Chem Lett
April 2024
Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, 20133 Milano, Italy.
Eumelanins play a crucial role as photoprotective agents for living organisms, yet the nature of the stationary and transient species involved in the light absorption and deactivation processes remains controversial. Moreover, the critical sub-100 fs time scale, which is key to the characterization of the primary excited species, has remained unexplored. Here, we study the eumelanin analogue polydopamine (PDA) and employ a combination of steady-state and transient optical spectroscopies to reveal the presence of spectrally broad coupled electronic transitions with, at least partial, charge-transfer (CT) character.
View Article and Find Full Text PDFHigh temporal resolution is essential for ultra-fast pump-probe experiments. Arrival time jitter and drift measurements, as well as their control, become critical especially when combining XUV or X-ray free-electron lasers (FELs) with optical lasers due to the large scale of such facilities and their distinct pulse generation processes. This paper presents the application of a laser pulse arrival time monitor that actively corrects the arrival time of an optical laser relative to the FEL's main optical clock.
View Article and Find Full Text PDFWe present a frequency domain, AOM-based pulse shaper that utilizes Brewster prisms rather than the current standard of gratings. In doing so, we demonstrate a three-fold increase in efficiency and the ability to compensate for temporal dispersion created by the acousto-optic modulator that filters the pulse spectrum. The shaper is tested between the wavelengths of 520-660 and 840-1170 nm, creating sub-50 fs pulses for each, and used to collect a 2D white-light spectrum of a thin film of semiconducting carbon nanotubes.
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