Aquatic ecosystems are major sources of greenhouse gases (GHG). Representative measurements of GHG fluxes from aquatic ecosystems to the atmosphere are vital for quantitative understanding of relationships between biogeochemistry and climate. Fluxes occur at high temporal variability at diel or longer scales, which are not captured by traditional short-term deployments (often in the order of 30 min) of floating flux chambers. High temporal frequency measurements are necessary but also extremely labor intensive if manual flux chamber based methods are used. Therefore, we designed an inexpensive and easily mobile automated flux chamber (AFC) for extended deployments. The AFC was designed to measure in situ accumulation of gas in the chamber and also to collect gas samples in an array of sample bottles for subsequent analysis in the laboratory, providing two independent ways of CH(4) concentration measurements. We here present the AFC design and function together with data from initial laboratory tests and from a field deployment.
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Sci Total Environ
January 2025
Department of Biology, Ecology and Earth Sciences (DIBEST), University of Calabria, Ponte Bucci street, cube 15B, 87036 Rende, Italy.
The work aims to estimate natural greenhouse gas emissions from soils in the Sibari Coastal Plain (Southern Italy), to understand (i) the contribution in terms of the total amount of CO and CH emitted in non-volcanic areas, (ii) the relationship among emitted gas, land use, organic matter and tectonic structures, and (iii) their potential environmental implications. Data were elaborated with statistical and geostatistical methods to separate the different populations and obtain prediction and probability maps. Methane fluxes had values consistently below the detection limit (0.
View Article and Find Full Text PDFMembranes (Basel)
January 2025
DVGW-Research Center at the Engler-Bunte-Institute, Water Chemistry and Water Technology, Karlsruhe Institute of Technology, Engler-Bunte-Ring 9, 76131 Karlsruhe, Germany.
Short-chain fatty acids (SCFAs) are valuable metabolic intermediates that are produced during dark fermentation of sludge, which, when capitalized on, can be used as chemical precursors for biotechnological applications. However, high concentrations of solids with SCFAs in hydrolyzed sludge can be highly detrimental to downstream recovery processes. This pilot-scale study addresses this limitation and explores the recovery of SCFAs from primary sludge into a particle-free permeate through a combination of chamber filter-press (material: polyester; mesh size: 100 µm) and cross-flow microfiltration (material: α-AlO; pore size: 0.
View Article and Find Full Text PDFEnviron Res
January 2025
China Academy of Safety Science and Technology, Beijing 100012, China. Electronic address:
Spontaneous coal fires are a significant source of greenhouse gas emissions, contributing to global warming. However, the lack of reliable estimation methods and research has obscured the full environmental impact of these emissions. This paper presents a novel quantification method for fugitive carbon emissions from spontaneous coal combustion.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
Associate Professor of Mechanical Engineering, College of Engineering, University of Georgia (UGA), 302 E. Campus Rd., Athens 30602, United States.
This study introduces a biomimetic approach to 3D printing multilayered hierarchical porous membranes (MHMs) using Direct Ink Writing (DIW) technology. Fabricated through a fast layer-by-layer printing process with varying concentrations of pore-forming agents, the produced MHMs mimic the hierarchical pore structure and filtration capabilities of natural soil systems. As a result, the 3D-printed MHMs achieved an impressive oil rejection rate of 99.
View Article and Find Full Text PDFSci Total Environ
January 2025
Department of Forest Sciences, Faculty of Agricultural and Environmental Sciences, Universidad de La Frontera, Temuco, Chile.
Peatlands are key ecosystems for global climate regulation because they provide the most efficient carbon sink on the planet. Despite this, they have been widely degraded by various anthropogenic disturbances, causing imbalances in their ecological functioning. A more recent type of disturbance corresponds to the commercial extraction of Sphagnum mosses, which has been carried out in temperate peatlands distributed in Australasia and Patagonia.
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