Assessment of ⁷Be content in precipitation in a South American semi-arid environment.

Sci Total Environ

Grupo de Estudios Ambientales, Instituto de Matemática Aplicada San Luis, Universidad Nacional de San Luis/CCT-San Luis-CONICET, San Luis, Argentina.

Published: December 2012

There are two naturally occurring radiogenic isotopes of beryllium, ⁷Be and ¹⁰Be. These are produced when cosmic radiation interacts with oxygen and nitrogen in the atmosphere. After production, these radionuclides are input to ecosystems through wet and dry deposition. In recent years ⁷Be and ¹⁰Be have proved to be powerful tools for studying dynamic processes that occur on the surface of the earth. We measured the ⁷Be content in precipitation at a semiarid location in central Argentina. From November 2006 to March 2009, 68 precipitation events were collected. Measured ⁷Be content ranged from 0.7±0.4 Bq L⁻¹ to 3.2±0.7 Bq L⁻¹, with a mean of 1.7 Bq L⁻¹ ±0.6 Bq L⁻¹. Beryllium-7 content of rainfall did not show clear relationships with amount of rainfall (mm), mean intensity (mm h⁻¹) or duration (h⁻¹), or elapsed time between events (day). The general results indicate that for the typical range of precipitation there was no atmospheric washout and that the reload of the atmosphere is not a relevant factor, but when the amount of precipitation is very high washout may occur. On the other hand, when the ⁷Be content was measured during single rain events, a high content of this radionuclide was found to be associated with very low rainfall intensity (≈3 mm h⁻¹), this suggests that rain intensity could affect the ⁷Be content. Using all data, a good linear relationship between ⁷Be deposition and rain magnitude was obtained (r²=0.82, p<0.0001). Because of this, the slope of this linear regression equation may be applied as a tool for tracing environmental processes that affect the surface of the earth. We can do this by directly estimating erosion/sedimentation processes using ⁷Be or by estimating the input of ¹⁰Be in the environment with the aim to evaluate land degradation phenomena.

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http://dx.doi.org/10.1016/j.scitotenv.2012.09.079DOI Listing

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