The lack of structural symmetry which usually characterizes semiconductor quantum dots lifts the energetic degeneracy of the bright excitonic states and hampers severely their use as high-fidelity sources of entangled photons. We demonstrate experimentally and theoretically that it is always possible to restore the excitonic degeneracy by the simultaneous application of large strain and electric fields. This is achieved by using one external perturbation to align the polarization of the exciton emission along the axis of the second perturbation, which then erases completely the energy splitting of the states. This result, which holds for any quantum dot structure, highlights the potential of combining complementary external fields to create artificial atoms meeting the stringent requirements posed by scalable semiconductor-based quantum technology.
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http://dx.doi.org/10.1103/PhysRevLett.109.147401 | DOI Listing |
Entropy (Basel)
October 2024
Research Institute CODE, University of the Bundeswehr Munich, 81739 Munich, Germany.
ACS Nano
July 2024
IBM Research Europe─Zurich, Säumerstrasse 4, 8803 Rüschlikon, Switzerland.
Nano Lett
April 2024
Laboratoire de Physique de l'École Normale Supérieure, ENS, Université PSL, CNRS, Sorbonne Université, Université Paris-Cité, F-75005 Paris, France.
Understanding the interplay between bright and dark exciton states is crucial for deciphering the luminescence properties of low-dimensional materials. The origin of the outstanding brightness of lead halide perovskites remains elusive. Here, we analyze temperature-dependent time-resolved photoluminescence to investigate the population mixing between bright and dark exciton sublevels in individual CsPbBr nanocrystals in the intermediate confinement regime.
View Article and Find Full Text PDFLight Sci Appl
October 2023
Université de Limoges XLIM UMR CNRS 7252, 123 Av. A. Thomas, 87060, Limoges, France.
The mid-infrared spectral region opens up new possibilities for applications such as molecular spectroscopy with high spatial and frequency resolution. For example, the mid-infrared light provided by synchrotron sources has helped for early diagnosis of several pathologies. However, alternative light sources at the table-top scale would enable better access to these state-of-the-art characterizations, eventually speeding up research in biology and medicine.
View Article and Find Full Text PDFNature
October 2023
National Astronomical Observatory of Japan, Tokyo, Japan.
During the first 500 million years of cosmic history, the first stars and galaxies formed, seeding the Universe with heavy elements and eventually reionizing the intergalactic medium. Observations with the James Webb Space Telescope (JWST) have uncovered a surprisingly high abundance of candidates for early star-forming galaxies, with distances (redshifts, z), estimated from multiband photometry, as large as z ≈ 16, far beyond pre-JWST limits. Although such photometric redshifts are generally robust, they can suffer from degeneracies and occasionally catastrophic errors.
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