The study of classical spins in topological insulators (Liu and Ma 2009 Phys. Rev. B 80 115216) is generalized to topological superconductors. Based on the characteristic features of the so-called F-function, the Bogoliubov-de Gennes Hamiltonian for superconductors is classified to positive, negative, and zero 'gap' categories for topologically trivial and nontrivial phases of a topological superconductor as well as a BCS superconductor, respectively. It is found that the F-function determines directly the presence or absence of localized excited states, induced by bulk classical spins and nonmagnetic impurities, in the superconducting gap and their persistence with respect to impurity strength. Our results provide an alternative way to identify topologically insulating and superconducting phases in experiments without resorting to the surface properties.
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http://dx.doi.org/10.1088/0953-8984/24/45/455701 | DOI Listing |
Phys Chem Chem Phys
January 2025
Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700 South Cass Avenue, Lemont, Illinois 60439, USA.
Photosynthetic reaction center proteins (RCs) provide ideal model systems for studying quantum entanglement between multiple spins, a quantum mechanical phenomenon wherein the properties of the entangled particles become inherently correlated. Following light-generated sequential electron transfer, RCs generate spin-correlated radical pairs (SCRPs), also referred to as entangled spin qubit (radical) pairs (SQPs). Understanding and controlling coherence mechanisms in SCRP/SQPs is important for realizing practical uses of electron spin qubits in quantum sensing applications.
View Article and Find Full Text PDFACS Nano
January 2025
Department of Physics, University of Basel, Klingelbergstrasse 82, 4056 Basel, Switzerland.
High-precision molecular manipulation techniques are used to control the distance between radical molecules on superconductors. Our results show that the molecules can host single electrons with a spin 1/2. By changing the distance between tip and sample, a quantum phase transition from the singlet to doublet ground state can be induced.
View Article and Find Full Text PDFLight Sci Appl
January 2025
Department of Physics, Chalmers University of Technology, 412 96, Gothenburg, Sweden.
Nanostructured dielectric metasurfaces offer unprecedented opportunities to control light-matter momentum exchange, and thereby the forces and torques that light can exert on matter. Here we introduce optical metasurfaces as components of ultracompact untethered microscopic metaspinners capable of efficient light-induced rotation in a liquid environment. Illuminated by weakly focused light, a metaspinner generates torque via photon recoil through the metasurfaces' ability to bend light towards high angles despite their sub-wavelength thickness, thereby creating orbital angular momentum.
View Article and Find Full Text PDFJ Phys Condens Matter
January 2025
CAMD, Computational Atomic-Scale Materials Design, Department of Physics, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark.
The magnetic properties of solids are typically analyzed in terms of Heisenberg models where the electronic structure is approximated by interacting localized spins. However, even in such models the evaluation of thermodynamic properties constitutes a major challenge and is usually handled by a mean field decoupling scheme. The random phase approximation (RPA) comprises a common approach and is often applied to evaluate critical temperatures although it is well known that the method is only accurate wellthe critical temperature.
View Article and Find Full Text PDFJ Sep Sci
December 2024
Institute of Pharmaceutical Sciences, Pharmaceutical (Bio-)Analysis, University of Tübingen, Tübingen, Germany.
The present work reports on the preparation, characterization, and evaluation of a set of novel triphenyl-modified silica-based stationary phases without and with embedded ion-exchange sites for mixed-mode liquid chromatography. The three synthesized triphenyl phases differed in additionally incorporated ion-exchange sites. In one embodiment, allyltriphenylsilane was bonded to thiol-modified silica by thiol-ene click reaction, leading to particles with no ion-exchange sites.
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