We report on the simultaneous observation of spontaneous symmetry breaking and long-range spatial coherence both in the strong- and the weak-coupling regime in a semiconductor microcavity. Under pulsed excitation, the formation of a stochastic order parameter is observed in polariton and photon lasing regimes. Single-shot measurements of the Stokes vector of the emission exhibit the buildup of stochastic polarization. Below threshold, the polarization noise does not exceed 10%, while above threshold we observe a total polarization of up to 50% after each excitation pulse, while the polarization averaged over the ensemble of pulses remains nearly zero. In both polariton and photon lasing regimes, the stochastic polarization buildup is accompanied by the buildup of spatial coherence. We find that the Landau criterion of spontaneous symmetry breaking and Penrose-Onsager criterion of long-range order for Bose-Einstein condensation are met in both polariton and photon lasing regimes.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1103/PhysRevLett.109.016404 | DOI Listing |
Nanophotonics
January 2025
Departamento de Ingeniería Electrónica, E.T.S.I. de Telecomunicación, Instituto de Sistemas Optoelectrónicos y Microtecnología (ISOM), Universidad Politécnica de Madrid, Madrid, 28040 Spain.
Polar biaxial crystals with extreme anisotropy hold promise for the spatial control and the manipulation of polaritons, as they can undergo topological transitions. However, taking advantage of these unique properties for nanophotonic devices requires to find mechanisms to modulate dynamically the material response. Here, we present a study on the propagation of surface phonon polaritons (SPhPs) in a photonic architecture based on a thin layer of α-MoO deposited on a semiconducting 4H-SiC substrate, whose carrier density can be tuned through photoinduction.
View Article and Find Full Text PDFNano Lett
January 2025
Department of Chemistry, University of Rochester, Rochester, New York 14627, United States.
Recent experiments have shown that exciton transport can be significantly enhanced through hybridization with confined photonic modes in a cavity. The light-matter hybridization generates exciton-polariton (EP) bands, whose group velocity is significantly larger than the excitons. Dissipative mechanisms that affect the constituent states of EPs, such as exciton-phonon coupling and cavity loss, have been observed to reduce the group velocities in experiments.
View Article and Find Full Text PDFACS Photonics
January 2025
Department of Physics, University of Pittsburgh, 3941 O'Hara Street, Pittsburgh, Pennsylvania 15218, United States.
We report the canonical properties of the Bose-Einstein condensation of polaritons in the weak coupling regime, seen previously in many low-temperature experiments, at room temperature in a GaAs/AlGaAs structure. These effects include a nonlinear energy shift of the polaritons, showing that they are not noninteracting photons, and dramatic line narrowing due to coherence, giving coherent emission with a spectral width of 0.24 meV at room temperature with no external stabilization.
View Article and Find Full Text PDFChem Commun (Camb)
January 2025
Research Institute for Electronic Science (RIES), Hokkaido University, N20W10, Kita ward, Hokkaido 001-0020, Japan.
Photochemical reactions enable the synthesis of energetically unfavorable compounds but often require irradiation with ultraviolet light, which potentially induces side reactions. Here, cavity strong coupling enhances the efficiency of an all-solid state photocyclization in crystals of 2,4-dimethoxy-β-nitrostyrene under irradiation with visible light. The exposure to visible light facilitates photocyclization by the transition to a lower polaritonic state, which is energetically lower than the original transition state.
View Article and Find Full Text PDFAdv Mater
January 2025
State Key Laboratory of Low-Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, 100084, P.R. China.
Over the past decade, semiconducting halide perovskite lasers have emerged as a transformative platform in optoelectronics, owing to unique properties such as high photoluminescence quantum yields, tunable bandgaps, and low-cost fabrication processes. This review systematically examines the advancements in halide perovskite lasers, covering diverse laser architectures, such as whispering gallery mode, Fabry-Pérot, plasmonic, bound states in the continuum (BIC), quantum dot, and polariton lasers. The mechanisms of optical gain, the role of material engineering in optimizing lasing performance, and the challenges associated with continuous-wave (CW) pumping and electrically driven lasing are discussed.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!