Theoretical description of quantum effects in multi-chromophoric aggregates.

Philos Trans A Math Phys Eng Sci

Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA 02139, USA.

Published: August 2012

AI Article Synopsis

  • Recent experiments indicate that excitations can move coherently within light-harvesting complexes, which are important for energy transfer in biological systems.
  • The discussion covers the evolution of theoretical models used to study this energy transfer, starting from the foundational models by Förster and Davydov.
  • The text also highlights modern theoretical approaches that build on these early models, reflecting advancements in understanding energy dynamics in molecular aggregates.

Article Abstract

Recent experiments on light-harvesting complexes have shown clear indication of coherent transport of excitations in these aggregates. We discuss the theoretical models that have been used to study energy transfer in molecular aggregates, beginning with the early models of Förster and Davydov and ending with the theoretical models of the present day.

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http://dx.doi.org/10.1098/rsta.2011.0204DOI Listing

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