The heavy fermion metal CeB(6) exhibits a hidden order of the antiferroquadrupolar (AFQ) type below T(Q)=3.2 K and a subsequent antiferromagnetic (AFM) order at T(N)=2.3 K. It was interpreted as an ordering of the quadrupole and dipole moments of a Γ(8) quartet of localized Ce 4f(1) electrons. This established picture has been profoundly shaken by recent inelastic neutron scattering (G. Friemel et al., arXiv:1111.4151) that found the evolution of a feedback spin exciton resonance within the hidden order phase at the AFQ wave vector which is stabilized by the AFM order. We develop an alternative theory based on a fourfold degenerate Anderson lattice model, including both order parameters as particle-hole condensates of itinerant heavy quasiparticles. This explains in a natural way the appearance of the spin exciton resonance and the momentum dependence of its spectral weight, in particular, around the AFQ vector and its rapid disappearance in the disordered phase. Analogies to the feedback effect in unconventional heavy fermion superconductors are pointed out.
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http://dx.doi.org/10.1103/PhysRevLett.108.146403 | DOI Listing |
Phys Rev Lett
December 2024
University of Michigan, Department of Physics, Ann Arbor, Michigan 48109, USA.
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Clermont INP, Institut Pascal, PHOTON-N2, Université Clermont Auvergne, CNRS, F-63000 Clermont-Ferrand, France.
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View Article and Find Full Text PDFACS Nano
January 2025
Beijing Academy of Quantum Information Sciences, Beijing 100193, P. R. China.
The quantum-well-like two-dimensional lead-halide perovskites exhibit strongly confined excitons due to the quantum confinement and reduced dielectric screening effect, which feature intriguing excitonic effects. The ionic nature of the perovskite crystal and the "softness" of the lattice induce the complex lattice dynamics. There are still open questions about how the soft lattices decorate the nature of excitons in these hybrid materials.
View Article and Find Full Text PDFJ Am Chem Soc
January 2025
Department of Chemistry, Graduate School of Science, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan.
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January 2025
Department of Chemistry and Biochemistry, George Mason University, Fairfax, Virginia 22030, United States.
The simulation of non-Markovian quantum dynamics plays an important role in the understanding of charge and exciton dynamics in the condensed phase environment, yet such a simulation remains computationally expensive on classical computers. In this work, we develop a variational quantum algorithm that is capable of simulating non-Markovian quantum dynamics on quantum computers. The algorithm captures the non-Markovian effect by employing the Ehrenfest trajectories and Monte Carlo sampling of their thermal distribution.
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