Using a Particle Environment Simulator, laboratory simulation experiment on the influence of resuspension on the release of mercury from sediments collected from medium tidal flat and low tidal flat in Chongming Dongtan was conducted. Results indicated that the conditions of overlying water changed significantly during resuspension. The concentrations of HgD and HgP were mainly in the rang of 0.152-2.657 microg x L(-1), 0.080-2.722 microg x L(-1) separately. In the resuspension processes, mercury was released from the medium intertidal sediments under the salinity condition of 4.1 per thousand, 8.0 per thousand, 10.0 per thousand, 13.0 per thousand, and from the low intertidal sediments under the salinity condition of 13.0 per thousand. However, the release of mercury from the medium intertidal sediments is not significant under the salinity condition of 4.1 per thousand, 8.0 per thousand, 10.0 per thousand. The salinity of overlying water had an important effect on resuspension. In different salinity condition, the release of mercury was different. And the release of mercury from medium tidal flat and low tidal flat was different during the resuspension periods, the release of mercury from the medium intertidal sediment was significantly higher than the release from the low intertidal sediment. When the rotate speed was (210 +/- 5) r x min(-1), the desorption of mercury significantly increased, thereby the rotate speed had an effect on the release of mercury.
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Nat Commun
January 2025
Department of Earth and Environmental Sciences, Tulane University, New Orleans, LA, 70118, USA.
Mercury (Hg) contamination poses a persistent threat to the remote Arctic ecosystem, yet the mechanisms driving the pronounced summer rebound of atmospheric gaseous elemental Hg (Hg) and its subsequent fate remain unclear due to limitations in large-scale seasonal studies. Here, we use an integrated atmosphere-land-sea-ice-ocean model to simulate Hg cycling in the Arctic comprehensively. Our results indicate that oceanic evasion is the dominant source (~80%) of the summer Hg rebound, particularly driven by seawater Hg release facilitated by seasonal ice melt (~42%), with further contributions from anthropogenic deposition and terrestrial re-emissions.
View Article and Find Full Text PDFEnviron Toxicol Chem
January 2025
Savannah River Ecology Lab, University of Georgia, Aiken, SC, USA.
Legacy contaminants tied to energy production are a worldwide concern. Coal combustion residues (CCRs) contain high concentrations of potentially toxic trace elements such as arsenic (As), mercury (Hg), and selenium (Se), which can persist for decades after initial contamination. CCR disposal methods, including aquatic settling basins and landfills, can facilitate environmental exposure through intentional and accidental releases.
View Article and Find Full Text PDFInt J Biol Macromol
January 2025
Beijing Key Laboratory of Ionic Liquids Clean Process, State Key Laboratory of Mesoscience and Engineering, CAS Key Laboratory of Green Process and Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China; School of Chemical Engineering, University of Chinese Academy of Sciences, Beijing 100049, China; Zhengzhou Institute of Emerging Industrial Technology, Zhengzhou 450000, China. Electronic address:
With the rising prevalence of lithium-ion batteries, efficient recovery of metal ions, particularly those potentially released from LiFePO anodes, has become critical. Given that both Fe and Li ions can form electrostatic adsorptive interactions, achieving effective separation of conventional adsorbent materials becomes challenging. This study presents an amino acid-functionalized nanocellulose hydrogel (ANH) synthesized by incorporating L-threonine, which significantly enhances the selective adsorption of Fe in a mixed-ion environment by leveraging coordination differences between Li and Fe.
View Article and Find Full Text PDFJ Hazard Mater
January 2025
Polish Academy of Sciences, Institute of Oceanology, Department of Marine Chemistry and Biochemistry, Powstańców Warszawy 55, Sopot 81-712, Poland.
Marine sediments are major sources of legacy pollution, capable of releasing toxic mercury (Hg) into the water column when disturbed. This study evaluated Hg remobilization from surface sediments during resuspension events by examining sediment properties, Hg concentrations, and speciation. Research was conducted in the southern Baltic Sea, representing diverse environmental conditions and human impacts.
View Article and Find Full Text PDFSci Total Environ
January 2025
Trent University, Peterborough, Ontario, Canada.
Arctic rivers may be the largest net sources of mercury (Hg) to the Arctic Ocean, yet riverine sources of Hg remain poorly characterized compared to atmospheric processes. This article reviews the current state of knowledge on Hg inputs to the Mackenzie River and Valley in Northern Canada from six point and non-point sources. Point sources include the locations of mines, fossil fuel extraction facilities, and retrogressive permafrost thaw slumps.
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