We report on the recovery of the short-range static magnetic order and on the concomitant degradation of the superconducting state in optimally F-doped SmFe(1-x)Ru(x)AsO(0.85)F(0.15) for 0.1≤x≲0.5. The two reduced order parameters coexist within nanometer-size domains in the FeAs layers and eventually disappear around a common critical threshold x(c)~0.6. Superconductivity and magnetism are shown to be closely related to two distinct well-defined local electronic environments of the FeAs layers. The two transition temperatures, controlled by the isoelectronic and diamagnetic Ru substitution, scale with the volume fraction of the corresponding environments. This fact indicates that superconductivity is assisted by magnetic fluctuations, which are frozen whenever a short-range static order appears, and totally vanish above the magnetic dilution threshold x(c).
Download full-text PDF |
Source |
|---|---|
| http://dx.doi.org/10.1103/PhysRevLett.107.227003 | DOI Listing |
Publication Analysis
Top Keywords
Similar Publications
Investigating the Origin of Automatic Rhodopsin Modeling Outliers Using the Microbial Rhodopsin as Testbed.
J Phys Chem B
December 2024
Aix Marseille Univ, CNRS, ICR, 13013 Marseille, France.
The automatic rhodopsin modeling (ARM) approach is a computational workflow devised for the automatic buildup of hybrid quantum mechanics/molecular mechanics (QM/MM) models of wild-type rhodopsins and mutants, with the purpose of establishing trends in their photophysical and photochemical properties. Despite the success of ARM in accurately describing the visible light absorption maxima of many rhodopsins, for a few cases, called outliers, it might lead to large deviations with respect to experiments. Applying ARM to rhodopsin (GR), a microbial rhodopsin with important applications in optogenetics, we analyze the origin of such outliers in the absorption energies obtained for GR wild-type and mutants at neutral pH, with a total root-mean-square deviation (RMSD) of 0.
View Article and Find Full Text PDFUnderstanding the superconductivity and charge density wave interaction through quasi-static lattice fluctuations.
Proc Natl Acad Sci U S A
December 2024
Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025.
In unconventional superconductors, coupled charge and lattice degrees of freedom can manifest in ordered phases of matter that are intertwined. In the cuprate family, fluctuating short-range charge correlations can coalesce into a longer-range charge density wave (CDW) order which is thought to intertwine with superconductivity, yet the nature of the interaction is still poorly understood. Here, by measuring subtle lattice fluctuations in underdoped YBaCuO on quasi-static timescales (thousands of seconds) through X-ray photon correlation spectroscopy, we report sensitivity to both superconductivity and CDW.
View Article and Find Full Text PDFAimed at addressing the problem of azimuth measurement of a short-range target with a pulsed laser, a new, to our knowledge, azimuth measurement method based on a single-pulse laser beam expanding mechanism is proposed based on the research of the pulse laser dynamic/static azimuth detection method. The echo power equation of single-pulse laser beam expanding short-range detection is derived theoretically. Combined with the spatial geometric distribution of the optical path and the normalized sum-difference angle measurement algorithm of the four-quadrant detector, a single-pulse laser short-range azimuth angle calculation model is established.
View Article and Find Full Text PDFUnique magnetic transition process demonstrating the effectiveness of bond percolation theory in a quantum magnet.
Nat Commun
November 2024
Department of Materials Science and Engineering, Graduate School of Engineering, Tohoku University, Sendai, Japan.
Like the crystallization of water to ice, magnetic transition occurs at a critical temperature after the slowing down of dynamically fluctuating short-range correlated spins. Here, we report a unique type of magnetic transition characterized by a linear increase in the volume fraction of unconventional static short-range-ordered spin clusters, which triggered a transition into a long-range order at a threshold fraction perfectly matching the bond percolation theory in a new quantum antiferromagnet of pseudo-trigonal Cu(OH)Cl. Static short-range order appeared in its Kagome lattice plane below ca.
View Article and Find Full Text PDFStructural Disorder of a Layered Lithium Manganese Oxide Cathode Paving a Reversible Phase Transition Route toward Its Theoretical Capacity.
J Am Chem Soc
December 2024
Department of Materials Science and Engineering, Korea University, Seoul 02841, Republic of Korea.
Layered lithium manganese oxides suffer from irreversible phase transitions induced by Mn migration and/or dissolution associated with the Jahn-Teller effect (JTE) of Mn, leading to inevitable capacity fading during cycling. The popular doping strategy of oxidizing Mn to Mn to relieve the JTE cannot completely eliminate the detrimental structural collapse from the cooperative JTE. Therefore, they are considered to be impractical for commercial use as cathode materials.
View Article and Find Full Text PDFWant AI Summaries of new PubMed Abstracts delivered to your In-box?
Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!