We have successfully grown ultrasmall cobalt nanostructures (lateral size below 30 nm) by optimization of the growth conditions using focused electron-beam-induced deposition techniques. This direct-write nanolithography technique is thus shown to produce unprecedented resolution in the growth of magnetic nanostructures. The challenging magnetic characterization of such small structures is here carried out by means of electron holography techniques. Apart from growing ultranarrow nanowires, very small Hall sensors have been created and their large response has been unveiled.
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http://dx.doi.org/10.1021/nn201517r | DOI Listing |
Beilstein J Nanotechnol
January 2025
Physics Institute, Goethe University Frankfurt, Max-von-Laue-Str. 1, 60438 Frankfurt am Main, Germany.
A fast simulation approach for focused electron beam induced deposition (FEBID) numerically solves the diffusion-reaction equation (continuum model) of the precursor surface on the growing nanostructure in conjunction with a Monte Carlo simulation for electron transport in the growing deposit. An important requirement in this regard is to have access to a methodology that can be used to systematically determine the values for the set of precursor parameters needed for this model. In this work we introduce such a method to derive the precursor sticking coefficient as one member of the precursor parameter set.
View Article and Find Full Text PDFMolecules
January 2025
Faculty of Chemistry, Nicolaus Copernicus University in Toruń, Gagarina 7, 87-100 Toruń, Poland.
We report the synthesis and characterization of new, user-friendly gold(I) [Au(μ-(NH)CCF)] coordination polymer and [AuCl(NH(NH=)CCF)] complex. These compounds were investigated for potential application as precursors in chemical vapor deposition (CVD) and focused electron/ion beam-induced deposition (FEBID/FIBID), which are additive methods to produce nanomaterials. Single-crystal X-ray diffraction, elemental analysis, and infrared spectroscopy were used to determine the complexes' composition and structure.
View Article and Find Full Text PDFJ Phys Condens Matter
November 2024
Institute of Applied Physics, Vienna University of Technology, Wiedner Hauptstr. 8-10/134, Wien, 1040, AUSTRIA.
The transition from planar (2D) to three-dimensional (3D) magnetic nanostructures represents a significant advancement in both fundamental research and practical applications, offering vast potential for next-generation technologies like ultrahigh-density storage, memory, logic, and neuromorphic computing. Despite being a relatively new field, the emergence of 3D nanomagnetism presents numerous opportunities for innovation, prompting the creation of a comprehensive roadmap by leading international researchers. This roadmap aims to facilitate collaboration and interdisciplinary dialogue to address challenges in materials science, physics, engineering, and computing.
View Article and Find Full Text PDFNanoscale Horiz
January 2025
Department of Material Science and Engineering, University of Tennessee - Knoxville, Knoxville, TN 37996, USA.
In this work, we explore focused electron beam induced etching (FEBIE) of niobium thin films with the XeF precursor as a route to edit, on-the-fly, superconducting devices. We report the effect of XeF pressure, electron beam current, beam energy, and dwell time on the Nb etch rate. To understand the mass transport and reaction rate limiting mechanisms, we compare the relative electron and XeF gas flux and reveal the process is reaction rate limited at low current/short dwell times, but shifts to mass transport limited regimes as both are increased.
View Article and Find Full Text PDFBeilstein J Nanotechnol
October 2024
Department of Nanometrology, Wrocław University of Science and Technology, Janiszewskiego 11/17, 50-370, Wrocław, Poland.
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