We develop a functional renormalization group approach which describes the low-energy single-particle properties of the Anderson impurity model up to intermediate on-site interactions [Formula: see text], where Δ is the hybridization in the wide-band limit. Our method is based on a generalization of a method proposed by Schütz et al (2005 Phys. Rev. B 72 035107), using two independent Hubbard-Stratonovich fields associated with transverse and longitudinal spin fluctuations. Although we do not reproduce the exponentially small Kondo scale in the limit [Formula: see text], the spin fluctuations included in our approach remove the unphysical Stoner instability predicted by mean field theory for U>πΔ. We discuss different decoupling schemes and show that a decoupling which manifestly respects the spin-rotational invariance of the problem gives rise to the lowest quasiparticle weight. To obtain a closed flow equation for the fermionic self-energy we also propose a new scheme of truncation of the functional renormalization group flow equations using Dyson-Schwinger equations to express bosonic vertex functions in terms of fermionic ones.
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http://dx.doi.org/10.1088/0953-8984/21/30/305602 | DOI Listing |
J Chem Phys
January 2025
Department of Chemistry, University of Waterloo, Waterloo, Ontario N2L 3G1, Canada.
Typical path integral Monte Carlo approaches use the primitive approximation to compute the probability density for a given path. In this work, we develop the pair discrete variable representation (pair-DVR) approach to study molecular rotations. The pair propagator, which was initially introduced to study superfluidity in condensed helium, is naturally well-suited for systems interacting with a pairwise potential.
View Article and Find Full Text PDFNano Lett
January 2025
Institute for Experimental and Applied Physics, University of Regensburg, 93040 Regensburg, Germany.
Understanding and controlling the electronic properties of two-dimensional materials are crucial for their potential applications in nano- and optoelectronics. Monolayer transition metal dichalcogenides have garnered significant interest due to their strong light-matter interaction and extreme sensitivity of the band structure to the presence of photogenerated electron-hole pairs. In this study, we investigate the transient electronic structure of monolayer WS on a graphene substrate after resonant excitation of the A-exciton using time- and angle-resolved photoemission spectroscopy.
View Article and Find Full Text PDFAm J Biol Anthropol
January 2025
Primate Models for Behavioural Evolution Lab, Institute of Human Sciences, University of Oxford, Oxford, UK.
Objectives: With contemporary, human-induced climate change at a crisis point, extreme weather events (e.g., cyclones, heatwaves, floods) are becoming more frequent, intense, and difficult to predict.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
II. Physikalisches Institut, Universität zu Köln, Zülpicher Straße 77, 50937 Cologne, Germany.
We report spin-polarized scanning tunneling microscopy measurements of an Anderson impurity system in MoS_{2} mirror-twin boundaries, where both the quantum-confined impurity state and the Kondo resonance resulting from the interaction with the substrate are accessible. Using a spin-polarized tip, we observe magnetic-field-induced changes in the peak heights of the Anderson impurity states as well as in the magnetic-field-split Kondo resonance. Quantitative comparison with numerical renormalization group calculations provides evidence of the notable spin polarization of the spin-resolved impurity spectral function under the influence of a magnetic field.
View Article and Find Full Text PDFNano Lett
January 2025
Wyant College of Optical Sciences, University of Arizona, 1630 East University Boulevard, Tucson, Arizona 85721, United States.
Microscopic many-body models based on inputs from first-principles density functional theory are used to calculate the carrier losses due to free carrier Auger-Meitner recombination (AMR) processes in Mo- and W-based monolayer transition metal dichalcogenides as a function of the carrier density, temperature, and dielectric environment. Despite the exceptional strength of Coulomb interaction in the two-dimensional materials, the AMR losses are found to be similar in magnitude to those in conventional III-V-based quantum wells for the same wavelengths. Unlike the case in III-V materials, the losses show nontrivial density dependencies due to the fact that bandgap renormalizations on the order of hundreds of millielectronvolts can bring higher bands into or out of resonance with the optimal energy level for the AMR transition, approximately one bandgap from the lowest band.
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