We investigate theoretically the Čerenkov-type second-harmonic generation in two-dimensional bulk nonlinear photonic crystal with longitudinal modulation of the χ((2)) nonlinearity. We show that in this scheme the Čerenkov radiation can be achieved simultaneously at multiple directions with comparable intensities. The angles of emission are controllable by the spatial modulation of the nonlinearity. We propose a design of the periodically poled domain pattern, which maximizes the efficiency of the second-harmonic emission.

Download full-text PDF

Source
http://dx.doi.org/10.1364/OL.36.002593DOI Listing

Publication Analysis

Top Keywords

second-harmonic generation
8
bulk nonlinear
8
nonlinear photonic
8
photonic crystal
8
tailoring Čerenkov
4
Čerenkov second-harmonic
4
generation bulk
4
crystal investigate
4
investigate theoretically
4
theoretically Čerenkov-type
4

Similar Publications

Finding novel efficient nonlinear optical materials with large second-order nonlinearity for the UV spectral range remains a formidable challenge, especially for silicate systems. Using a high-temperature solid reaction in a tight vacuum environment, two ultraviolet nonlinear optical materials with a moderate second harmonic generation (SHG) response have been created: PbSiOC and PbCaSiO. The SHG values they computed are roughly 2.

View Article and Find Full Text PDF

Organic-inorganic hybrid lead halides have been extensively studied due to their outstanding physical properties and diverse compositional elements. However, environmentally benign tin-based hybrids with remarkable flexibility in bandgap engineering have been less investigated. Herein, we report the successful design and synthesis of three tin-based organic-inorganic hybrid compounds through precise molecular modification: [Me(i-Pr)N][SnBr] (), [MeCHCl(i-Pr)N][SnBr] (), and [MeCHBr(i-Pr-Br)N][SnBr] ().

View Article and Find Full Text PDF

Symmetry Breaking in Twisted Mixed-Dimensional Heterostructure Interfaces for Multifunctional Polarization-Sensitive Photodetection.

ACS Nano

January 2025

Center for High Pressure Science (CHiPS), State Key Laboratory of Metastable Materials Science & Technology, Yanshan University, Qinhuangdao 066004, China.

Moiré superlattices, created by stacking different van der Waals materials at twist angles, have emerged as a versatile platform for exploring intriguing phenomena such as topological properties, superconductivity, the quantum anomalous Hall effect, and the unconventional Stark effect. Additionally, the formation of moiré superlattice potential can generate spontaneous symmetry breaking, leading to an anisotropic optical response and electronic transport behavior. Herein, we propose a two-step chemical vapor deposition (CVD) strategy for synthesizing WS/SbS moiré superlattices.

View Article and Find Full Text PDF

Cantilever-Enhanced Fiber-Optic Photoacoustic Spectrophone for Low-Pressure Gas Detection.

Anal Chem

January 2025

School of Optoelectronic Engineering and Instrumentation Science, Dalian University of Technology, Dalian 116024, Liaoning, China.

A cantilever-enhanced fiber-optic photoacoustic (PA) spectrophone is reported for trace gas detection at a low-pressure environment. A cantilever-based fiber-optic Fabry-Perot (F-P) interferometer (FPI) is utilized for simultaneous measurement of air pressure and PA pressure. Since the cantilever resonance frequency follows air pressure linearly, the fundamental frequency intensity modulation (1-IM) technique is applied to scan the frequency response of the solid PA signal from tube wall absorption for tracking the cantilever resonance frequency in real time.

View Article and Find Full Text PDF

Two Alkaline Metal Borates: from Layer to Layer-Pillared Framework.

Inorg Chem

December 2024

MOE Key Laboratory of Cluster Science, School of Chemistry and Chemical Engineering, Beijing Institute of Technology, Beijing 102488, China.

Two borates, NaK[BO(OH)]·HO () and NaK[{BO}{BO}{BO(OH)}]·2HO () have been designed and made under solvothermal conditions. Compound exhibits a 2D fluctuant layer based on the [BO(OH)] clusters, containing two types of 9-membered ring (MR) channels and showing a four-connected sql topology net. By modifying the reactants and reaction temperature, compound was obtained from compound .

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!