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A triad [FeFe] hydrogenase system for light-driven hydrogen evolution. | LitMetric
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A triad [FeFe] hydrogenase system for light-driven hydrogen evolution.

Hong-Yan Wang Gang Si Wei-Ning Cao Wen-Guang Wang Zhi-Jun Li Feng Wang Chen-Ho Tung Li-Zhu Wu

Chem Commun (Camb)

Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry & Graduate University, Chinese Academy of Sciences, Beijing 100190, PR China.

Published: August 2011

A novel molecular triad [FeFe]-H(2)ase 1, and its model complexes 2 and 3 have been successfully constructed. The multistep PET and long-lived Fe(i)Fe(0) species were found to be responsible for the better performance of triad 1 than that of 2 with 3 for light-driven H(2) evolution.

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 Source
http://dx.doi.org/10.1039/c1cc12200bDOI Listing

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