Ferromagnetic resonance is the most widely used technique for characterizing ferromagnetic materials. However, its use is generally restricted to wafer-scale samples or specific micro-magnetic devices, such as spin valves, which have a spatially varying magnetization profile and where ferromagnetic resonance can be induced by an alternating current owing to angular momentum transfer. Here we introduce a form of ferromagnetic resonance in which an electric current oscillating at microwave frequencies is used to create an effective magnetic field in the magnetic material being probed, which makes it possible to characterize individual nanoscale samples with uniform magnetization profiles. The technique takes advantage of the microscopic non-collinearity of individual electron spins arising from spin-orbit coupling and bulk or structural inversion asymmetry in the band structure of the sample. We characterize lithographically patterned (Ga,Mn)As and (Ga,Mn)(As,P) nanoscale bars, including broadband measurements of resonant damping as a function of frequency, and measurements of anisotropy as a function of bar width and strain. In addition, vector magnetometry on the driving fields reveals contributions with the symmetry of both the Dresselhaus and Rashba spin-orbit interactions.
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http://dx.doi.org/10.1038/nnano.2011.68 | DOI Listing |
ACS Nano
January 2025
Department of Bioengineering, University of Pennsylvania, 210 S. 33rd Street, 435 Skirkanich Hall, Philadelphia, Pennsylvania 19104, United States.
Nanoparticles have gained attention as drug delivery vehicles for cancer treatment, but often struggle with poor tumor accumulation and penetration. Single external magnets can enhance magnetic nanoparticle delivery but are limited to superficial tumors due to the rapid decline in the magnetic field strength with distance. We previously showed that a 2-magnet device could extend targeting to greater tissue depths.
View Article and Find Full Text PDFNat Commun
January 2025
New Cornerstone Science Laboratory, Department of Physics, University of Hong Kong, 999077, Hong Kong, China.
Tellegen medium has long been a topic of debate, with its existence being contested over several decades. It was first proposed by Tellegen in 1948 and is characterized by a real-valued cross coupling between electric and magnetic responses, distinguishing it from the well-known chiral medium that has imaginary coupling coefficients. Significantly, Tellegen responses are closely linked to axion dynamics, an extensively studied subject in condensed matter physics.
View Article and Find Full Text PDFACS Cent Sci
December 2024
Division of Chemistry and Chemical Engineering, Arthur Amos Noyes Laboratory of Chemical Physics, California Institute of Technology, Pasadena, California 91125, United States.
Spin-lattice relaxation constitutes a key challenge for the development of quantum technologies, as it destroys superpositions in molecular quantum bits (qubits) and magnetic memory in single molecule magnets (SMMs). Gaining mechanistic insight into the spin relaxation process has proven challenging owing to a lack of spectroscopic observables and contradictions among theoretical models. Here, we use pulse electron paramagnetic resonance (EPR) to profile changes in spin relaxation rates ( ) as a function of both temperature and magnetic field orientation, forming a two-dimensional data matrix.
View Article and Find Full Text PDFSmall
December 2024
Department of Applied Physics and Center of Quantum Materials and Devices, Chongqing University, Chongqing, 401331, China.
The observation of both resonant quantum tunneling of magnetization (RQTM) and resonant quantum magnetodielectric (RQMD) effect in the perovskite multiferroic metal-organic framework [CHNH]Co(HCOO).is reported. An intrinsic magnetic phase separation emerges at low temperatures due to the hydrogen-bond-modified long-range super-exchange interaction, leading to the coexistence of canted antiferromagnetic order and single-ion (Co) magnets.
View Article and Find Full Text PDFIn this Letter, we calculate the optical and magneto-optical reflectivity in a dielectric/gap/ferromagnet excited by a -polarized monochromatic optical beam through the prism (Otto configuration) as a function of the angle of incidence and the gap thickness . Besides the well-known surface plasmon polariton (SPP resonance at ∼ ), we find a new, to the best of our knowledge, resonance with a nanometric gap ∼ 10 nm at a large ∼ 80°. Both resonances display pronounced resonant behavior in the transverse magneto-optical Kerr effect (T-MOKE).
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